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Efficient Non-Linear Optical Spectroscopy with Multiple High-Frequency Modulated Optical Frequency Combs

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Abstract

A novel non-linear spectroscopy with multiple high-frequency modulated optical frequency combs that is capable of high S/N detection of the non-linear polarization of a system is theoretically derived and analyzed. This detection of the nonlinear optical signature essentially bypasses interference due to the background laser fields and is achieved by obtaining a component of the observed polarization as spikes in the field-free region between consecutive comb-lines. Related experiments have been designed and effective polarization due to such sources have been successfully obtained.

© 2018 The Author(s)

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