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Towards an all-purpose laser excitation tool for multimodal nonlinear microscopy

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Abstract

Nonlinear spectroscopic methods and in particular the combination of several nonlinear optical modalities in one setup, such as coherent Raman microscopy, second harmonic generation or two-photon fluorescence, have seen tremendous development over the recent years resulting in many different applications in both the material and life sciences. In this contribution we discuss the experimental realization of a novel concept for multimodal nonlinear microscopy which combines ultrashort, sub 10 fs laser pulses with pulse shapers (Fig.1a), and show in detail the successful implementation of adaptive spectral focussing schemes for Raman and Mid-IR spectroscopy and other coherently controlled nonlinear processes.

© 2018 The Author(s)

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