Expand this Topic clickable element to expand a topic
Skip to content
Optica Publishing Group

Diagonal slice four-wave mixing: natural separation of coherent broadening mechanisms

Abstract

We present an ultrafast coherent spectroscopy data acquisition scheme that samples slices of the time domain used in multidimensional coherent spectroscopy to achieve faster data collection than full spectra. We derive analytical expressions for resonance lineshapes using this technique that completely separate homogeneous and inhomogeneous broadening contributions into separate projected lineshapes for arbitrary inhomogeneous broadening. These lineshape expressions are also valid for slices taken from full multidimensional spectra and allow direct measurement of the parameters contributing to the lineshapes in those spectra as well as our own.

© 2018 Optical Society of America

Full Article  |  PDF Article
More Like This
Analytical calculation of two-dimensional spectra

Joshua D. Bell, Rebecca Conrad, and Mark E. Siemens
Opt. Lett. 40(7) 1157-1160 (2015)

Absolute phase calibration in phase-modulated multidimensional coherent spectroscopy

Geoffrey M. Diederich and Mark E. Siemens
Opt. Lett. 44(12) 3054-3057 (2019)

Resonance lineshapes in two-dimensional Fourier transform spectroscopy

Mark E. Siemens, Galan Moody, Hebin Li, Alan D. Bristow, and Steven T. Cundiff
Opt. Express 18(17) 17699-17708 (2010)

Cited By

You do not have subscription access to this journal. Cited by links are available to subscribers only. You may subscribe either as an Optica member, or as an authorized user of your institution.

Contact your librarian or system administrator
or
Login to access Optica Member Subscription

Figures (3)

You do not have subscription access to this journal. Figure files are available to subscribers only. You may subscribe either as an Optica member, or as an authorized user of your institution.

Contact your librarian or system administrator
or
Login to access Optica Member Subscription

Equations (8)

You do not have subscription access to this journal. Equations are available to subscribers only. You may subscribe either as an Optica member, or as an authorized user of your institution.

Contact your librarian or system administrator
or
Login to access Optica Member Subscription

Select as filters


Select Topics Cancel
© Copyright 2024 | Optica Publishing Group. All Rights Reserved