Abstract

Bismuth-doped materials show fascinating near-infrared (NIR) photoluminescence (PL) properties. However, synthesizing Bi-doped, NIR-luminescent, nanometer-sized materials with high PL quantum yields remains challenging. Here, Bi-doped CsPbI3 perovskite nanocrystals (NCs) with an average size less than 10 nm and showing a superbroad NIR PL covering the telecommunication and second biological optical windows were achieved. The NIR PL quantum yield of these NCs is up to 7.17% with the Bi doping concentration of 0.074%. Additionally, efficient energy transfer from the semiconducting CsPbI3 to bismuth-related active center can be realized. We anticipate that the developed systems may find applications in optoelectronic and photonic devices as well as biological imaging. This work enriches the bank of Bi-doped luminescent materials, and might stimulate research interest for synthesizing other classes of Bi-activated nanomaterials.

© 2017 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

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References

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    [Crossref]
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    [Crossref]
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    [Crossref] [PubMed]
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    [Crossref] [PubMed]
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2017 (1)

Y. Zhou, Z.-J. Yong, W. Zhang, J.-P. Ma, A. Sadhanala, Y.-M. Chen, B.-M. Liu, Y. Zhou, B. Song, and H.-T. Sun, “Ultra-broadband optical amplification at telecommunication wavelengths achieved by bismuth-activated lead iodide perovskites,” J. Mater. Chem. C Mater. Opt. Electron. Devices 5(10), 2591–2596 (2017).
[Crossref]

2016 (7)

Y. Zhou, D.-D. Zhou, B.-M. Liu, L.-N. Li, Z.-J. Yong, H. Xing, Y.-Z. Fang, J.-S. Hou, and H.-T. Sun, “Ultrabroad near-infrared photoluminescence from bismuth doped CsPbI3: polaronic defects vs. bismuth active centers,” J. Mater. Chem. C Mater. Opt. Electron. Devices 4(12), 2295–2301 (2016).
[Crossref]

S. Gu, B. Zhou, W. Luo, L. Wang, W. Jiang, W. Jiang, and J. Ballato, “Near-infrared broadband photoluminescence of bismuth-doped zeolite-derived silica glass prepared by SPS,” J. Am. Ceram. Soc. 99(1), 121–127 (2016).
[Crossref]

S. Lin, X. Zhang, P. Zhang, D. Tan, J. Xu, W. Li, and K. Chen, “High-efficiency near-infrared emission from Bismuth-doped SiO0.73 thin films fabricated by ion implantation technology,” Opt. Lett. 41(3), 630–633 (2016).
[Crossref] [PubMed]

B. M. Liu, Z. G. Zhang, K. Zhang, Y. Kuroiwa, C. Moriyoshi, H. M. Yu, C. Li, L. R. Zheng, L. N. Li, G. Yang, Y. Zhou, Y. Z. Fang, J. S. Hou, Y. Matsushita, and H. T. Sun, “Unconventional luminescent centers in metastable phases created by topochemical reduction reactions,” Angew. Chem. Int. Ed. Engl. 55(16), 4967–4971 (2016).
[Crossref] [PubMed]

B. Saparov and D. B. Mitzi, “Organic-inorganic perovskites: structural versatility for functional materials design,” Chem. Rev. 116(7), 4558–4596 (2016).
[Crossref] [PubMed]

Y. Zhou, Z. J. Yong, K. C. Zhang, B. M. Liu, Z. W. Wang, J. S. Hou, Y. Z. Fang, Y. Zhou, H. T. Sun, and B. Song, “Ultrabroad Photoluminescence and Electroluminescence at New Wavelengths from Doped Organometal Halide Perovskites,” J. Phys. Chem. Lett. 7(14), 2735–2741 (2016).
[Crossref] [PubMed]

X. Li, Y. Wu, S. Zhang, B. Cai, Y. Gu, J. Song, and H. Zeng, “CsPbX3 Quantum Dots for Lighting and Displays: Room Temperature Synthesis, Photoluminescence Superiorities, Underlying Origins and White Light-Emitting Diodes,” Adv. Funct. Mater. 26(15), 2435–2445 (2016).
[Crossref]

2015 (3)

L. Protesescu, S. Yakunin, M. I. Bodnarchuk, F. Krieg, R. Caputo, C. H. Hendon, R. X. Yang, A. Walsh, and M. V. Kovalenko, “Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut,” Nano Lett. 15(6), 3692–3696 (2015).
[Crossref] [PubMed]

O. Laguta, H. E. Hamzaoui, M. Bouazaoui, V. B. Arion, and I. Razdobreev, “Anti-Stokes photoluminescence in Ga/Bi co-doped sol-gel silica glass,” Opt. Lett. 40(7), 1591–1594 (2015).
[Crossref] [PubMed]

Y. Wang, X. Li, J. Song, L. Xiao, H. Zeng, and H. Sun, “All-Inorganic Colloidal Perovskite Quantum Dots: A New Class of Lasing Materials with Favorable Characteristics,” Adv. Mater. 27(44), 7101–7108 (2015).
[Crossref] [PubMed]

2014 (1)

H.-T. Sun, J. Zhou, and J. Qiu, Prog. “Recent advances in bismuth activated photonic materials,” Prog. Mater. Sci. 64(10), 1–72 (2014).
[Crossref]

2013 (2)

B. B. Xu, S. F. Zhou, D. Z. Tan, Z. L. Hong, J. H. Hao, and J. R. Qiu, “Multifunctional tunable ultra-broadband visible and near-infrared luminescence from bismuth-doped germanate glasses,” J. Appl. Phys. 113(8), 083503 (2013).
[Crossref]

B. Xu, J. Hao, S. Zhou, and J. Qiu, “Ultra-broadband infrared luminescence of Bi-doped thin-films for integrated optics,” Opt. Express 21(15), 18532–18537 (2013).
[Crossref] [PubMed]

2012 (5)

L. Su, H. Zhao, H. Li, L. Zhang, X. Fan, X. Jiang, H. Tang, G. Ren, J. Xu, W. R-Romanowski, R. Lisiecki, and P. solarz, “Near-infrared photoluminescence spectra in Bi doped CsI crystal: Evidence for Bi-valence conversions and Bi ion,” Opt. Mater. Express 2(6), 757–764 (2012).
[Crossref]

B. Xu, D. Tan, S. Zhou, Z. Hong, K. N. Sharafudeen, and J. Qiu, “Enhanced broadband near-infrared luminescence of Bi-doped oxyfluoride glasses,” Opt. Express 20(27), 29105–29111 (2012).
[Crossref] [PubMed]

C. Li, Z. Song, J. Qiu, Z. Yang, X. Yu, D. Zhou, Z. Yin, R. Wang, Y. Xu, and Y. Cao, “Broadband yellow–white and near infrared luminescence from Bi-doped Ba10(PO4)6Cl2 prepared in reductive atmosphere,” J. Lumin. 132(7), 1807–1811 (2012).
[Crossref]

A. A. Veber, A. N. Romanov, O. V. Usovich, Z. T. Fattakhova, E. V. Haula, V. N. Korchak, L. A. Trusov, P. E. Kazin, V. B. Sulimov, and V. B. Tsvetkov, “Luminescent properties of Bi-doped polycrystalline KAlCl4,” Appl. Phys. B 108(4), 733–736 (2012).
[Crossref]

E. M. Dianov, “Bismuth-doped optical fibers: a challenging active medium for near-IR lasers and optical amplifiers,” Light Sci. Appl. 1(5), e12 (2012).
[Crossref]

2011 (6)

H. T. Sun, J. Yang, M. Fujii, Y. Sakka, Y. Zhu, T. Asahara, N. Shirahata, M. Ii, Z. Bai, J. G. Li, and H. Gao, “Highly fluorescent silica-coated bismuth-doped aluminosilicate nanoparticles for near-infrared bioimaging,” Small 7(2), 199–203 (2011).
[Crossref] [PubMed]

D. Mocatta, G. Cohen, J. Schattner, O. Millo, E. Rabani, and U. Banin, “Heavily doped semiconductor nanocrystal quantum dots,” Science 332(6025), 77–81 (2011).
[Crossref] [PubMed]

H.-T. Sun, Y. Sakka, H. Gao, Y. Miwa, M. Fujii, N. Shirahata, Z. Bai, and J.-G. Li, “Ultrabroad near-infrared photoluminescence from Bi5(AlCl4)3 crystal,” J. Mater. Chem. 21(12), 4060–4063 (2011).
[Crossref]

A. N. Romanov, E. V. Haula, Z. T. Fattakhova, A. A. Veber, V. B. Tsvetkov, D. M. Zhigunov, V. N. Korchak, and V. B. Sulimov, “Near-IR luminescence from subvalent bismuth species in fluoride glass,” Opt. Mater. 34(1), 155–158 (2011).
[Crossref]

H.-T. Sun, Y. Sakka, M. Fujii, N. Shirahata, and H. Gao, “Ultrabroad near-infrared photoluminescence from ionic liquids containing subvalent bismuth,” Opt. Lett. 36(2), 100–102 (2011).
[Crossref] [PubMed]

L. Su, H. Zhao, H. Li, L. Zheng, G. Ren, J. Xu, W. Ryba-Romanowski, R. Lisiecki, and P. Solarz, “Near-infrared ultrabroadband luminescence spectra properties of subvalent bismuth in CsI halide crystals,” Opt. Lett. 36(23), 4551–4553 (2011).
[Crossref] [PubMed]

2010 (3)

2009 (2)

L. Su, J. Yu, P. Zhou, H. Li, L. Zheng, Y. Yang, F. Wu, H. Xia, and J. Xu, “Broadband near-infrared luminescence in γ-irradiated Bi-doped α-BaB2O4 single crystals,” Opt. Lett. 34(16), 2504–2506 (2009).
[Crossref] [PubMed]

H.-T. Sun, A. Hosokawa, Y. Miwa, F. Shimaoka, M. Fujii, M. Mizuhata, S. Hayashi, and S. Deki, “Strong ultra-broadband near-infrared photoluminescence from bismuth-embedded zeolites and their derivatives,” Adv. Mater. 21(36), 3694–3698 (2009).
[Crossref]

2008 (1)

1997 (1)

J. C. de Mello, H. F. Wittmann, and R. H. Friend, “An Improved Experimental Determination of External Photoluminescence Quantum Efficiency,” Adv. Mater. 9(3), 230–232 (1997).
[Crossref]

Arion, V. B.

Asahara, T.

H. T. Sun, J. Yang, M. Fujii, Y. Sakka, Y. Zhu, T. Asahara, N. Shirahata, M. Ii, Z. Bai, J. G. Li, and H. Gao, “Highly fluorescent silica-coated bismuth-doped aluminosilicate nanoparticles for near-infrared bioimaging,” Small 7(2), 199–203 (2011).
[Crossref] [PubMed]

Bai, Z.

H. T. Sun, J. Yang, M. Fujii, Y. Sakka, Y. Zhu, T. Asahara, N. Shirahata, M. Ii, Z. Bai, J. G. Li, and H. Gao, “Highly fluorescent silica-coated bismuth-doped aluminosilicate nanoparticles for near-infrared bioimaging,” Small 7(2), 199–203 (2011).
[Crossref] [PubMed]

H.-T. Sun, Y. Sakka, H. Gao, Y. Miwa, M. Fujii, N. Shirahata, Z. Bai, and J.-G. Li, “Ultrabroad near-infrared photoluminescence from Bi5(AlCl4)3 crystal,” J. Mater. Chem. 21(12), 4060–4063 (2011).
[Crossref]

Ballato, J.

S. Gu, B. Zhou, W. Luo, L. Wang, W. Jiang, W. Jiang, and J. Ballato, “Near-infrared broadband photoluminescence of bismuth-doped zeolite-derived silica glass prepared by SPS,” J. Am. Ceram. Soc. 99(1), 121–127 (2016).
[Crossref]

Banin, U.

D. Mocatta, G. Cohen, J. Schattner, O. Millo, E. Rabani, and U. Banin, “Heavily doped semiconductor nanocrystal quantum dots,” Science 332(6025), 77–81 (2011).
[Crossref] [PubMed]

Bodnarchuk, M. I.

L. Protesescu, S. Yakunin, M. I. Bodnarchuk, F. Krieg, R. Caputo, C. H. Hendon, R. X. Yang, A. Walsh, and M. V. Kovalenko, “Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut,” Nano Lett. 15(6), 3692–3696 (2015).
[Crossref] [PubMed]

Boldyrev, K. N.

Bouazaoui, M.

Butvina, L. N.

Cai, B.

X. Li, Y. Wu, S. Zhang, B. Cai, Y. Gu, J. Song, and H. Zeng, “CsPbX3 Quantum Dots for Lighting and Displays: Room Temperature Synthesis, Photoluminescence Superiorities, Underlying Origins and White Light-Emitting Diodes,” Adv. Funct. Mater. 26(15), 2435–2445 (2016).
[Crossref]

Cao, Y.

C. Li, Z. Song, J. Qiu, Z. Yang, X. Yu, D. Zhou, Z. Yin, R. Wang, Y. Xu, and Y. Cao, “Broadband yellow–white and near infrared luminescence from Bi-doped Ba10(PO4)6Cl2 prepared in reductive atmosphere,” J. Lumin. 132(7), 1807–1811 (2012).
[Crossref]

Capoen, B.

Caputo, R.

L. Protesescu, S. Yakunin, M. I. Bodnarchuk, F. Krieg, R. Caputo, C. H. Hendon, R. X. Yang, A. Walsh, and M. V. Kovalenko, “Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut,” Nano Lett. 15(6), 3692–3696 (2015).
[Crossref] [PubMed]

Chen, K.

Chen, Y.-M.

Y. Zhou, Z.-J. Yong, W. Zhang, J.-P. Ma, A. Sadhanala, Y.-M. Chen, B.-M. Liu, Y. Zhou, B. Song, and H.-T. Sun, “Ultra-broadband optical amplification at telecommunication wavelengths achieved by bismuth-activated lead iodide perovskites,” J. Mater. Chem. C Mater. Opt. Electron. Devices 5(10), 2591–2596 (2017).
[Crossref]

Cohen, G.

D. Mocatta, G. Cohen, J. Schattner, O. Millo, E. Rabani, and U. Banin, “Heavily doped semiconductor nanocrystal quantum dots,” Science 332(6025), 77–81 (2011).
[Crossref] [PubMed]

de Mello, J. C.

J. C. de Mello, H. F. Wittmann, and R. H. Friend, “An Improved Experimental Determination of External Photoluminescence Quantum Efficiency,” Adv. Mater. 9(3), 230–232 (1997).
[Crossref]

Deki, S.

H.-T. Sun, A. Hosokawa, Y. Miwa, F. Shimaoka, M. Fujii, M. Mizuhata, S. Hayashi, and S. Deki, “Strong ultra-broadband near-infrared photoluminescence from bismuth-embedded zeolites and their derivatives,” Adv. Mater. 21(36), 3694–3698 (2009).
[Crossref]

Dianov, E. M.

E. M. Dianov, “Bismuth-doped optical fibers: a challenging active medium for near-IR lasers and optical amplifiers,” Light Sci. Appl. 1(5), e12 (2012).
[Crossref]

A. G. Okhrimchuk, L. N. Butvina, E. M. Dianov, N. V. Lichkova, V. N. Zagorodnev, and K. N. Boldyrev, “Near-infrared luminescence of RbPb2Cl5:Bi crystals,” Opt. Lett. 33(19), 2182–2184 (2008).
[Crossref] [PubMed]

El Hamzaoui, H.

Fan, X.

Fang, Y. Z.

Y. Zhou, Z. J. Yong, K. C. Zhang, B. M. Liu, Z. W. Wang, J. S. Hou, Y. Z. Fang, Y. Zhou, H. T. Sun, and B. Song, “Ultrabroad Photoluminescence and Electroluminescence at New Wavelengths from Doped Organometal Halide Perovskites,” J. Phys. Chem. Lett. 7(14), 2735–2741 (2016).
[Crossref] [PubMed]

B. M. Liu, Z. G. Zhang, K. Zhang, Y. Kuroiwa, C. Moriyoshi, H. M. Yu, C. Li, L. R. Zheng, L. N. Li, G. Yang, Y. Zhou, Y. Z. Fang, J. S. Hou, Y. Matsushita, and H. T. Sun, “Unconventional luminescent centers in metastable phases created by topochemical reduction reactions,” Angew. Chem. Int. Ed. Engl. 55(16), 4967–4971 (2016).
[Crossref] [PubMed]

Fang, Y.-Z.

Y. Zhou, D.-D. Zhou, B.-M. Liu, L.-N. Li, Z.-J. Yong, H. Xing, Y.-Z. Fang, J.-S. Hou, and H.-T. Sun, “Ultrabroad near-infrared photoluminescence from bismuth doped CsPbI3: polaronic defects vs. bismuth active centers,” J. Mater. Chem. C Mater. Opt. Electron. Devices 4(12), 2295–2301 (2016).
[Crossref]

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A. A. Veber, A. N. Romanov, O. V. Usovich, Z. T. Fattakhova, E. V. Haula, V. N. Korchak, L. A. Trusov, P. E. Kazin, V. B. Sulimov, and V. B. Tsvetkov, “Luminescent properties of Bi-doped polycrystalline KAlCl4,” Appl. Phys. B 108(4), 733–736 (2012).
[Crossref]

A. N. Romanov, E. V. Haula, Z. T. Fattakhova, A. A. Veber, V. B. Tsvetkov, D. M. Zhigunov, V. N. Korchak, and V. B. Sulimov, “Near-IR luminescence from subvalent bismuth species in fluoride glass,” Opt. Mater. 34(1), 155–158 (2011).
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J. C. de Mello, H. F. Wittmann, and R. H. Friend, “An Improved Experimental Determination of External Photoluminescence Quantum Efficiency,” Adv. Mater. 9(3), 230–232 (1997).
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H. T. Sun, J. Yang, M. Fujii, Y. Sakka, Y. Zhu, T. Asahara, N. Shirahata, M. Ii, Z. Bai, J. G. Li, and H. Gao, “Highly fluorescent silica-coated bismuth-doped aluminosilicate nanoparticles for near-infrared bioimaging,” Small 7(2), 199–203 (2011).
[Crossref] [PubMed]

H.-T. Sun, Y. Sakka, H. Gao, Y. Miwa, M. Fujii, N. Shirahata, Z. Bai, and J.-G. Li, “Ultrabroad near-infrared photoluminescence from Bi5(AlCl4)3 crystal,” J. Mater. Chem. 21(12), 4060–4063 (2011).
[Crossref]

H.-T. Sun, Y. Sakka, M. Fujii, N. Shirahata, and H. Gao, “Ultrabroad near-infrared photoluminescence from ionic liquids containing subvalent bismuth,” Opt. Lett. 36(2), 100–102 (2011).
[Crossref] [PubMed]

H.-T. Sun, F. Shimaoka, Y. Miwa, J. Ruan, M. Fujii, J. Qiu, and S. Hayashi, “Sensitized superbroadband near-IR emission in bismuth glass/Si nanocrystal superlattices,” Opt. Lett. 35(13), 2215–2217 (2010).
[Crossref] [PubMed]

H.-T. Sun, A. Hosokawa, Y. Miwa, F. Shimaoka, M. Fujii, M. Mizuhata, S. Hayashi, and S. Deki, “Strong ultra-broadband near-infrared photoluminescence from bismuth-embedded zeolites and their derivatives,” Adv. Mater. 21(36), 3694–3698 (2009).
[Crossref]

Gao, H.

H.-T. Sun, Y. Sakka, H. Gao, Y. Miwa, M. Fujii, N. Shirahata, Z. Bai, and J.-G. Li, “Ultrabroad near-infrared photoluminescence from Bi5(AlCl4)3 crystal,” J. Mater. Chem. 21(12), 4060–4063 (2011).
[Crossref]

H. T. Sun, J. Yang, M. Fujii, Y. Sakka, Y. Zhu, T. Asahara, N. Shirahata, M. Ii, Z. Bai, J. G. Li, and H. Gao, “Highly fluorescent silica-coated bismuth-doped aluminosilicate nanoparticles for near-infrared bioimaging,” Small 7(2), 199–203 (2011).
[Crossref] [PubMed]

H.-T. Sun, Y. Sakka, M. Fujii, N. Shirahata, and H. Gao, “Ultrabroad near-infrared photoluminescence from ionic liquids containing subvalent bismuth,” Opt. Lett. 36(2), 100–102 (2011).
[Crossref] [PubMed]

Gu, S.

S. Gu, B. Zhou, W. Luo, L. Wang, W. Jiang, W. Jiang, and J. Ballato, “Near-infrared broadband photoluminescence of bismuth-doped zeolite-derived silica glass prepared by SPS,” J. Am. Ceram. Soc. 99(1), 121–127 (2016).
[Crossref]

Gu, Y.

X. Li, Y. Wu, S. Zhang, B. Cai, Y. Gu, J. Song, and H. Zeng, “CsPbX3 Quantum Dots for Lighting and Displays: Room Temperature Synthesis, Photoluminescence Superiorities, Underlying Origins and White Light-Emitting Diodes,” Adv. Funct. Mater. 26(15), 2435–2445 (2016).
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Hao, J.

Hao, J. H.

B. B. Xu, S. F. Zhou, D. Z. Tan, Z. L. Hong, J. H. Hao, and J. R. Qiu, “Multifunctional tunable ultra-broadband visible and near-infrared luminescence from bismuth-doped germanate glasses,” J. Appl. Phys. 113(8), 083503 (2013).
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A. A. Veber, A. N. Romanov, O. V. Usovich, Z. T. Fattakhova, E. V. Haula, V. N. Korchak, L. A. Trusov, P. E. Kazin, V. B. Sulimov, and V. B. Tsvetkov, “Luminescent properties of Bi-doped polycrystalline KAlCl4,” Appl. Phys. B 108(4), 733–736 (2012).
[Crossref]

A. N. Romanov, E. V. Haula, Z. T. Fattakhova, A. A. Veber, V. B. Tsvetkov, D. M. Zhigunov, V. N. Korchak, and V. B. Sulimov, “Near-IR luminescence from subvalent bismuth species in fluoride glass,” Opt. Mater. 34(1), 155–158 (2011).
[Crossref]

Hayashi, S.

H.-T. Sun, F. Shimaoka, Y. Miwa, J. Ruan, M. Fujii, J. Qiu, and S. Hayashi, “Sensitized superbroadband near-IR emission in bismuth glass/Si nanocrystal superlattices,” Opt. Lett. 35(13), 2215–2217 (2010).
[Crossref] [PubMed]

H.-T. Sun, A. Hosokawa, Y. Miwa, F. Shimaoka, M. Fujii, M. Mizuhata, S. Hayashi, and S. Deki, “Strong ultra-broadband near-infrared photoluminescence from bismuth-embedded zeolites and their derivatives,” Adv. Mater. 21(36), 3694–3698 (2009).
[Crossref]

Hendon, C. H.

L. Protesescu, S. Yakunin, M. I. Bodnarchuk, F. Krieg, R. Caputo, C. H. Hendon, R. X. Yang, A. Walsh, and M. V. Kovalenko, “Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut,” Nano Lett. 15(6), 3692–3696 (2015).
[Crossref] [PubMed]

Hong, Z.

Hong, Z. L.

B. B. Xu, S. F. Zhou, D. Z. Tan, Z. L. Hong, J. H. Hao, and J. R. Qiu, “Multifunctional tunable ultra-broadband visible and near-infrared luminescence from bismuth-doped germanate glasses,” J. Appl. Phys. 113(8), 083503 (2013).
[Crossref]

Hosokawa, A.

H.-T. Sun, A. Hosokawa, Y. Miwa, F. Shimaoka, M. Fujii, M. Mizuhata, S. Hayashi, and S. Deki, “Strong ultra-broadband near-infrared photoluminescence from bismuth-embedded zeolites and their derivatives,” Adv. Mater. 21(36), 3694–3698 (2009).
[Crossref]

Hou, J. S.

Y. Zhou, Z. J. Yong, K. C. Zhang, B. M. Liu, Z. W. Wang, J. S. Hou, Y. Z. Fang, Y. Zhou, H. T. Sun, and B. Song, “Ultrabroad Photoluminescence and Electroluminescence at New Wavelengths from Doped Organometal Halide Perovskites,” J. Phys. Chem. Lett. 7(14), 2735–2741 (2016).
[Crossref] [PubMed]

B. M. Liu, Z. G. Zhang, K. Zhang, Y. Kuroiwa, C. Moriyoshi, H. M. Yu, C. Li, L. R. Zheng, L. N. Li, G. Yang, Y. Zhou, Y. Z. Fang, J. S. Hou, Y. Matsushita, and H. T. Sun, “Unconventional luminescent centers in metastable phases created by topochemical reduction reactions,” Angew. Chem. Int. Ed. Engl. 55(16), 4967–4971 (2016).
[Crossref] [PubMed]

Hou, J.-S.

Y. Zhou, D.-D. Zhou, B.-M. Liu, L.-N. Li, Z.-J. Yong, H. Xing, Y.-Z. Fang, J.-S. Hou, and H.-T. Sun, “Ultrabroad near-infrared photoluminescence from bismuth doped CsPbI3: polaronic defects vs. bismuth active centers,” J. Mater. Chem. C Mater. Opt. Electron. Devices 4(12), 2295–2301 (2016).
[Crossref]

Ii, M.

H. T. Sun, J. Yang, M. Fujii, Y. Sakka, Y. Zhu, T. Asahara, N. Shirahata, M. Ii, Z. Bai, J. G. Li, and H. Gao, “Highly fluorescent silica-coated bismuth-doped aluminosilicate nanoparticles for near-infrared bioimaging,” Small 7(2), 199–203 (2011).
[Crossref] [PubMed]

Ivanov, V. Y.

Jiang, W.

S. Gu, B. Zhou, W. Luo, L. Wang, W. Jiang, W. Jiang, and J. Ballato, “Near-infrared broadband photoluminescence of bismuth-doped zeolite-derived silica glass prepared by SPS,” J. Am. Ceram. Soc. 99(1), 121–127 (2016).
[Crossref]

S. Gu, B. Zhou, W. Luo, L. Wang, W. Jiang, W. Jiang, and J. Ballato, “Near-infrared broadband photoluminescence of bismuth-doped zeolite-derived silica glass prepared by SPS,” J. Am. Ceram. Soc. 99(1), 121–127 (2016).
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Jiang, X.

Kazin, P. E.

A. A. Veber, A. N. Romanov, O. V. Usovich, Z. T. Fattakhova, E. V. Haula, V. N. Korchak, L. A. Trusov, P. E. Kazin, V. B. Sulimov, and V. B. Tsvetkov, “Luminescent properties of Bi-doped polycrystalline KAlCl4,” Appl. Phys. B 108(4), 733–736 (2012).
[Crossref]

Korchak, V. N.

A. A. Veber, A. N. Romanov, O. V. Usovich, Z. T. Fattakhova, E. V. Haula, V. N. Korchak, L. A. Trusov, P. E. Kazin, V. B. Sulimov, and V. B. Tsvetkov, “Luminescent properties of Bi-doped polycrystalline KAlCl4,” Appl. Phys. B 108(4), 733–736 (2012).
[Crossref]

A. N. Romanov, E. V. Haula, Z. T. Fattakhova, A. A. Veber, V. B. Tsvetkov, D. M. Zhigunov, V. N. Korchak, and V. B. Sulimov, “Near-IR luminescence from subvalent bismuth species in fluoride glass,” Opt. Mater. 34(1), 155–158 (2011).
[Crossref]

Kovalenko, M. V.

L. Protesescu, S. Yakunin, M. I. Bodnarchuk, F. Krieg, R. Caputo, C. H. Hendon, R. X. Yang, A. Walsh, and M. V. Kovalenko, “Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut,” Nano Lett. 15(6), 3692–3696 (2015).
[Crossref] [PubMed]

Krieg, F.

L. Protesescu, S. Yakunin, M. I. Bodnarchuk, F. Krieg, R. Caputo, C. H. Hendon, R. X. Yang, A. Walsh, and M. V. Kovalenko, “Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut,” Nano Lett. 15(6), 3692–3696 (2015).
[Crossref] [PubMed]

Kuroiwa, Y.

B. M. Liu, Z. G. Zhang, K. Zhang, Y. Kuroiwa, C. Moriyoshi, H. M. Yu, C. Li, L. R. Zheng, L. N. Li, G. Yang, Y. Zhou, Y. Z. Fang, J. S. Hou, Y. Matsushita, and H. T. Sun, “Unconventional luminescent centers in metastable phases created by topochemical reduction reactions,” Angew. Chem. Int. Ed. Engl. 55(16), 4967–4971 (2016).
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Kustov, E. F.

Laguta, O.

Li, C.

B. M. Liu, Z. G. Zhang, K. Zhang, Y. Kuroiwa, C. Moriyoshi, H. M. Yu, C. Li, L. R. Zheng, L. N. Li, G. Yang, Y. Zhou, Y. Z. Fang, J. S. Hou, Y. Matsushita, and H. T. Sun, “Unconventional luminescent centers in metastable phases created by topochemical reduction reactions,” Angew. Chem. Int. Ed. Engl. 55(16), 4967–4971 (2016).
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C. Li, Z. Song, J. Qiu, Z. Yang, X. Yu, D. Zhou, Z. Yin, R. Wang, Y. Xu, and Y. Cao, “Broadband yellow–white and near infrared luminescence from Bi-doped Ba10(PO4)6Cl2 prepared in reductive atmosphere,” J. Lumin. 132(7), 1807–1811 (2012).
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Li, H.

Li, J. G.

H. T. Sun, J. Yang, M. Fujii, Y. Sakka, Y. Zhu, T. Asahara, N. Shirahata, M. Ii, Z. Bai, J. G. Li, and H. Gao, “Highly fluorescent silica-coated bismuth-doped aluminosilicate nanoparticles for near-infrared bioimaging,” Small 7(2), 199–203 (2011).
[Crossref] [PubMed]

Li, J.-G.

H.-T. Sun, Y. Sakka, H. Gao, Y. Miwa, M. Fujii, N. Shirahata, Z. Bai, and J.-G. Li, “Ultrabroad near-infrared photoluminescence from Bi5(AlCl4)3 crystal,” J. Mater. Chem. 21(12), 4060–4063 (2011).
[Crossref]

Li, L. N.

B. M. Liu, Z. G. Zhang, K. Zhang, Y. Kuroiwa, C. Moriyoshi, H. M. Yu, C. Li, L. R. Zheng, L. N. Li, G. Yang, Y. Zhou, Y. Z. Fang, J. S. Hou, Y. Matsushita, and H. T. Sun, “Unconventional luminescent centers in metastable phases created by topochemical reduction reactions,” Angew. Chem. Int. Ed. Engl. 55(16), 4967–4971 (2016).
[Crossref] [PubMed]

Li, L.-N.

Y. Zhou, D.-D. Zhou, B.-M. Liu, L.-N. Li, Z.-J. Yong, H. Xing, Y.-Z. Fang, J.-S. Hou, and H.-T. Sun, “Ultrabroad near-infrared photoluminescence from bismuth doped CsPbI3: polaronic defects vs. bismuth active centers,” J. Mater. Chem. C Mater. Opt. Electron. Devices 4(12), 2295–2301 (2016).
[Crossref]

Li, W.

Li, X.

X. Li, Y. Wu, S. Zhang, B. Cai, Y. Gu, J. Song, and H. Zeng, “CsPbX3 Quantum Dots for Lighting and Displays: Room Temperature Synthesis, Photoluminescence Superiorities, Underlying Origins and White Light-Emitting Diodes,” Adv. Funct. Mater. 26(15), 2435–2445 (2016).
[Crossref]

Y. Wang, X. Li, J. Song, L. Xiao, H. Zeng, and H. Sun, “All-Inorganic Colloidal Perovskite Quantum Dots: A New Class of Lasing Materials with Favorable Characteristics,” Adv. Mater. 27(44), 7101–7108 (2015).
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Lin, S.

Lisiecki, R.

Liu, B. M.

B. M. Liu, Z. G. Zhang, K. Zhang, Y. Kuroiwa, C. Moriyoshi, H. M. Yu, C. Li, L. R. Zheng, L. N. Li, G. Yang, Y. Zhou, Y. Z. Fang, J. S. Hou, Y. Matsushita, and H. T. Sun, “Unconventional luminescent centers in metastable phases created by topochemical reduction reactions,” Angew. Chem. Int. Ed. Engl. 55(16), 4967–4971 (2016).
[Crossref] [PubMed]

Y. Zhou, Z. J. Yong, K. C. Zhang, B. M. Liu, Z. W. Wang, J. S. Hou, Y. Z. Fang, Y. Zhou, H. T. Sun, and B. Song, “Ultrabroad Photoluminescence and Electroluminescence at New Wavelengths from Doped Organometal Halide Perovskites,” J. Phys. Chem. Lett. 7(14), 2735–2741 (2016).
[Crossref] [PubMed]

Liu, B.-M.

Y. Zhou, Z.-J. Yong, W. Zhang, J.-P. Ma, A. Sadhanala, Y.-M. Chen, B.-M. Liu, Y. Zhou, B. Song, and H.-T. Sun, “Ultra-broadband optical amplification at telecommunication wavelengths achieved by bismuth-activated lead iodide perovskites,” J. Mater. Chem. C Mater. Opt. Electron. Devices 5(10), 2591–2596 (2017).
[Crossref]

Y. Zhou, D.-D. Zhou, B.-M. Liu, L.-N. Li, Z.-J. Yong, H. Xing, Y.-Z. Fang, J.-S. Hou, and H.-T. Sun, “Ultrabroad near-infrared photoluminescence from bismuth doped CsPbI3: polaronic defects vs. bismuth active centers,” J. Mater. Chem. C Mater. Opt. Electron. Devices 4(12), 2295–2301 (2016).
[Crossref]

Luo, W.

S. Gu, B. Zhou, W. Luo, L. Wang, W. Jiang, W. Jiang, and J. Ballato, “Near-infrared broadband photoluminescence of bismuth-doped zeolite-derived silica glass prepared by SPS,” J. Am. Ceram. Soc. 99(1), 121–127 (2016).
[Crossref]

Ma, J.-P.

Y. Zhou, Z.-J. Yong, W. Zhang, J.-P. Ma, A. Sadhanala, Y.-M. Chen, B.-M. Liu, Y. Zhou, B. Song, and H.-T. Sun, “Ultra-broadband optical amplification at telecommunication wavelengths achieved by bismuth-activated lead iodide perovskites,” J. Mater. Chem. C Mater. Opt. Electron. Devices 5(10), 2591–2596 (2017).
[Crossref]

Matsushita, Y.

B. M. Liu, Z. G. Zhang, K. Zhang, Y. Kuroiwa, C. Moriyoshi, H. M. Yu, C. Li, L. R. Zheng, L. N. Li, G. Yang, Y. Zhou, Y. Z. Fang, J. S. Hou, Y. Matsushita, and H. T. Sun, “Unconventional luminescent centers in metastable phases created by topochemical reduction reactions,” Angew. Chem. Int. Ed. Engl. 55(16), 4967–4971 (2016).
[Crossref] [PubMed]

Millo, O.

D. Mocatta, G. Cohen, J. Schattner, O. Millo, E. Rabani, and U. Banin, “Heavily doped semiconductor nanocrystal quantum dots,” Science 332(6025), 77–81 (2011).
[Crossref] [PubMed]

Mitzi, D. B.

B. Saparov and D. B. Mitzi, “Organic-inorganic perovskites: structural versatility for functional materials design,” Chem. Rev. 116(7), 4558–4596 (2016).
[Crossref] [PubMed]

Miwa, Y.

H.-T. Sun, Y. Sakka, H. Gao, Y. Miwa, M. Fujii, N. Shirahata, Z. Bai, and J.-G. Li, “Ultrabroad near-infrared photoluminescence from Bi5(AlCl4)3 crystal,” J. Mater. Chem. 21(12), 4060–4063 (2011).
[Crossref]

H.-T. Sun, F. Shimaoka, Y. Miwa, J. Ruan, M. Fujii, J. Qiu, and S. Hayashi, “Sensitized superbroadband near-IR emission in bismuth glass/Si nanocrystal superlattices,” Opt. Lett. 35(13), 2215–2217 (2010).
[Crossref] [PubMed]

H.-T. Sun, A. Hosokawa, Y. Miwa, F. Shimaoka, M. Fujii, M. Mizuhata, S. Hayashi, and S. Deki, “Strong ultra-broadband near-infrared photoluminescence from bismuth-embedded zeolites and their derivatives,” Adv. Mater. 21(36), 3694–3698 (2009).
[Crossref]

Mizuhata, M.

H.-T. Sun, A. Hosokawa, Y. Miwa, F. Shimaoka, M. Fujii, M. Mizuhata, S. Hayashi, and S. Deki, “Strong ultra-broadband near-infrared photoluminescence from bismuth-embedded zeolites and their derivatives,” Adv. Mater. 21(36), 3694–3698 (2009).
[Crossref]

Mocatta, D.

D. Mocatta, G. Cohen, J. Schattner, O. Millo, E. Rabani, and U. Banin, “Heavily doped semiconductor nanocrystal quantum dots,” Science 332(6025), 77–81 (2011).
[Crossref] [PubMed]

Moriyoshi, C.

B. M. Liu, Z. G. Zhang, K. Zhang, Y. Kuroiwa, C. Moriyoshi, H. M. Yu, C. Li, L. R. Zheng, L. N. Li, G. Yang, Y. Zhou, Y. Z. Fang, J. S. Hou, Y. Matsushita, and H. T. Sun, “Unconventional luminescent centers in metastable phases created by topochemical reduction reactions,” Angew. Chem. Int. Ed. Engl. 55(16), 4967–4971 (2016).
[Crossref] [PubMed]

Okhrimchuk, A. G.

Protesescu, L.

L. Protesescu, S. Yakunin, M. I. Bodnarchuk, F. Krieg, R. Caputo, C. H. Hendon, R. X. Yang, A. Walsh, and M. V. Kovalenko, “Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut,” Nano Lett. 15(6), 3692–3696 (2015).
[Crossref] [PubMed]

Qiu, J.

Qiu, J. R.

B. B. Xu, S. F. Zhou, D. Z. Tan, Z. L. Hong, J. H. Hao, and J. R. Qiu, “Multifunctional tunable ultra-broadband visible and near-infrared luminescence from bismuth-doped germanate glasses,” J. Appl. Phys. 113(8), 083503 (2013).
[Crossref]

Rabani, E.

D. Mocatta, G. Cohen, J. Schattner, O. Millo, E. Rabani, and U. Banin, “Heavily doped semiconductor nanocrystal quantum dots,” Science 332(6025), 77–81 (2011).
[Crossref] [PubMed]

Razdobreev, I.

Ren, G.

Romanov, A. N.

A. A. Veber, A. N. Romanov, O. V. Usovich, Z. T. Fattakhova, E. V. Haula, V. N. Korchak, L. A. Trusov, P. E. Kazin, V. B. Sulimov, and V. B. Tsvetkov, “Luminescent properties of Bi-doped polycrystalline KAlCl4,” Appl. Phys. B 108(4), 733–736 (2012).
[Crossref]

A. N. Romanov, E. V. Haula, Z. T. Fattakhova, A. A. Veber, V. B. Tsvetkov, D. M. Zhigunov, V. N. Korchak, and V. B. Sulimov, “Near-IR luminescence from subvalent bismuth species in fluoride glass,” Opt. Mater. 34(1), 155–158 (2011).
[Crossref]

R-Romanowski, W.

Ruan, J.

Ryba-Romanowski, W.

Sadhanala, A.

Y. Zhou, Z.-J. Yong, W. Zhang, J.-P. Ma, A. Sadhanala, Y.-M. Chen, B.-M. Liu, Y. Zhou, B. Song, and H.-T. Sun, “Ultra-broadband optical amplification at telecommunication wavelengths achieved by bismuth-activated lead iodide perovskites,” J. Mater. Chem. C Mater. Opt. Electron. Devices 5(10), 2591–2596 (2017).
[Crossref]

Sakka, Y.

H.-T. Sun, Y. Sakka, H. Gao, Y. Miwa, M. Fujii, N. Shirahata, Z. Bai, and J.-G. Li, “Ultrabroad near-infrared photoluminescence from Bi5(AlCl4)3 crystal,” J. Mater. Chem. 21(12), 4060–4063 (2011).
[Crossref]

H. T. Sun, J. Yang, M. Fujii, Y. Sakka, Y. Zhu, T. Asahara, N. Shirahata, M. Ii, Z. Bai, J. G. Li, and H. Gao, “Highly fluorescent silica-coated bismuth-doped aluminosilicate nanoparticles for near-infrared bioimaging,” Small 7(2), 199–203 (2011).
[Crossref] [PubMed]

H.-T. Sun, Y. Sakka, M. Fujii, N. Shirahata, and H. Gao, “Ultrabroad near-infrared photoluminescence from ionic liquids containing subvalent bismuth,” Opt. Lett. 36(2), 100–102 (2011).
[Crossref] [PubMed]

Saparov, B.

B. Saparov and D. B. Mitzi, “Organic-inorganic perovskites: structural versatility for functional materials design,” Chem. Rev. 116(7), 4558–4596 (2016).
[Crossref] [PubMed]

Schattner, J.

D. Mocatta, G. Cohen, J. Schattner, O. Millo, E. Rabani, and U. Banin, “Heavily doped semiconductor nanocrystal quantum dots,” Science 332(6025), 77–81 (2011).
[Crossref] [PubMed]

Sharafudeen, K. N.

Shimaoka, F.

H.-T. Sun, F. Shimaoka, Y. Miwa, J. Ruan, M. Fujii, J. Qiu, and S. Hayashi, “Sensitized superbroadband near-IR emission in bismuth glass/Si nanocrystal superlattices,” Opt. Lett. 35(13), 2215–2217 (2010).
[Crossref] [PubMed]

H.-T. Sun, A. Hosokawa, Y. Miwa, F. Shimaoka, M. Fujii, M. Mizuhata, S. Hayashi, and S. Deki, “Strong ultra-broadband near-infrared photoluminescence from bismuth-embedded zeolites and their derivatives,” Adv. Mater. 21(36), 3694–3698 (2009).
[Crossref]

Shirahata, N.

H.-T. Sun, Y. Sakka, H. Gao, Y. Miwa, M. Fujii, N. Shirahata, Z. Bai, and J.-G. Li, “Ultrabroad near-infrared photoluminescence from Bi5(AlCl4)3 crystal,” J. Mater. Chem. 21(12), 4060–4063 (2011).
[Crossref]

H. T. Sun, J. Yang, M. Fujii, Y. Sakka, Y. Zhu, T. Asahara, N. Shirahata, M. Ii, Z. Bai, J. G. Li, and H. Gao, “Highly fluorescent silica-coated bismuth-doped aluminosilicate nanoparticles for near-infrared bioimaging,” Small 7(2), 199–203 (2011).
[Crossref] [PubMed]

H.-T. Sun, Y. Sakka, M. Fujii, N. Shirahata, and H. Gao, “Ultrabroad near-infrared photoluminescence from ionic liquids containing subvalent bismuth,” Opt. Lett. 36(2), 100–102 (2011).
[Crossref] [PubMed]

solarz, P.

Song, B.

Y. Zhou, Z.-J. Yong, W. Zhang, J.-P. Ma, A. Sadhanala, Y.-M. Chen, B.-M. Liu, Y. Zhou, B. Song, and H.-T. Sun, “Ultra-broadband optical amplification at telecommunication wavelengths achieved by bismuth-activated lead iodide perovskites,” J. Mater. Chem. C Mater. Opt. Electron. Devices 5(10), 2591–2596 (2017).
[Crossref]

Y. Zhou, Z. J. Yong, K. C. Zhang, B. M. Liu, Z. W. Wang, J. S. Hou, Y. Z. Fang, Y. Zhou, H. T. Sun, and B. Song, “Ultrabroad Photoluminescence and Electroluminescence at New Wavelengths from Doped Organometal Halide Perovskites,” J. Phys. Chem. Lett. 7(14), 2735–2741 (2016).
[Crossref] [PubMed]

Song, J.

X. Li, Y. Wu, S. Zhang, B. Cai, Y. Gu, J. Song, and H. Zeng, “CsPbX3 Quantum Dots for Lighting and Displays: Room Temperature Synthesis, Photoluminescence Superiorities, Underlying Origins and White Light-Emitting Diodes,” Adv. Funct. Mater. 26(15), 2435–2445 (2016).
[Crossref]

Y. Wang, X. Li, J. Song, L. Xiao, H. Zeng, and H. Sun, “All-Inorganic Colloidal Perovskite Quantum Dots: A New Class of Lasing Materials with Favorable Characteristics,” Adv. Mater. 27(44), 7101–7108 (2015).
[Crossref] [PubMed]

Song, Z.

C. Li, Z. Song, J. Qiu, Z. Yang, X. Yu, D. Zhou, Z. Yin, R. Wang, Y. Xu, and Y. Cao, “Broadband yellow–white and near infrared luminescence from Bi-doped Ba10(PO4)6Cl2 prepared in reductive atmosphere,” J. Lumin. 132(7), 1807–1811 (2012).
[Crossref]

Su, L.

Sulimov, V. B.

A. A. Veber, A. N. Romanov, O. V. Usovich, Z. T. Fattakhova, E. V. Haula, V. N. Korchak, L. A. Trusov, P. E. Kazin, V. B. Sulimov, and V. B. Tsvetkov, “Luminescent properties of Bi-doped polycrystalline KAlCl4,” Appl. Phys. B 108(4), 733–736 (2012).
[Crossref]

A. N. Romanov, E. V. Haula, Z. T. Fattakhova, A. A. Veber, V. B. Tsvetkov, D. M. Zhigunov, V. N. Korchak, and V. B. Sulimov, “Near-IR luminescence from subvalent bismuth species in fluoride glass,” Opt. Mater. 34(1), 155–158 (2011).
[Crossref]

Sun, H.

Y. Wang, X. Li, J. Song, L. Xiao, H. Zeng, and H. Sun, “All-Inorganic Colloidal Perovskite Quantum Dots: A New Class of Lasing Materials with Favorable Characteristics,” Adv. Mater. 27(44), 7101–7108 (2015).
[Crossref] [PubMed]

Sun, H. T.

B. M. Liu, Z. G. Zhang, K. Zhang, Y. Kuroiwa, C. Moriyoshi, H. M. Yu, C. Li, L. R. Zheng, L. N. Li, G. Yang, Y. Zhou, Y. Z. Fang, J. S. Hou, Y. Matsushita, and H. T. Sun, “Unconventional luminescent centers in metastable phases created by topochemical reduction reactions,” Angew. Chem. Int. Ed. Engl. 55(16), 4967–4971 (2016).
[Crossref] [PubMed]

Y. Zhou, Z. J. Yong, K. C. Zhang, B. M. Liu, Z. W. Wang, J. S. Hou, Y. Z. Fang, Y. Zhou, H. T. Sun, and B. Song, “Ultrabroad Photoluminescence and Electroluminescence at New Wavelengths from Doped Organometal Halide Perovskites,” J. Phys. Chem. Lett. 7(14), 2735–2741 (2016).
[Crossref] [PubMed]

H. T. Sun, J. Yang, M. Fujii, Y. Sakka, Y. Zhu, T. Asahara, N. Shirahata, M. Ii, Z. Bai, J. G. Li, and H. Gao, “Highly fluorescent silica-coated bismuth-doped aluminosilicate nanoparticles for near-infrared bioimaging,” Small 7(2), 199–203 (2011).
[Crossref] [PubMed]

Sun, H.-T.

Y. Zhou, Z.-J. Yong, W. Zhang, J.-P. Ma, A. Sadhanala, Y.-M. Chen, B.-M. Liu, Y. Zhou, B. Song, and H.-T. Sun, “Ultra-broadband optical amplification at telecommunication wavelengths achieved by bismuth-activated lead iodide perovskites,” J. Mater. Chem. C Mater. Opt. Electron. Devices 5(10), 2591–2596 (2017).
[Crossref]

Y. Zhou, D.-D. Zhou, B.-M. Liu, L.-N. Li, Z.-J. Yong, H. Xing, Y.-Z. Fang, J.-S. Hou, and H.-T. Sun, “Ultrabroad near-infrared photoluminescence from bismuth doped CsPbI3: polaronic defects vs. bismuth active centers,” J. Mater. Chem. C Mater. Opt. Electron. Devices 4(12), 2295–2301 (2016).
[Crossref]

H.-T. Sun, J. Zhou, and J. Qiu, Prog. “Recent advances in bismuth activated photonic materials,” Prog. Mater. Sci. 64(10), 1–72 (2014).
[Crossref]

H.-T. Sun, Y. Sakka, H. Gao, Y. Miwa, M. Fujii, N. Shirahata, Z. Bai, and J.-G. Li, “Ultrabroad near-infrared photoluminescence from Bi5(AlCl4)3 crystal,” J. Mater. Chem. 21(12), 4060–4063 (2011).
[Crossref]

H.-T. Sun, Y. Sakka, M. Fujii, N. Shirahata, and H. Gao, “Ultrabroad near-infrared photoluminescence from ionic liquids containing subvalent bismuth,” Opt. Lett. 36(2), 100–102 (2011).
[Crossref] [PubMed]

H.-T. Sun, F. Shimaoka, Y. Miwa, J. Ruan, M. Fujii, J. Qiu, and S. Hayashi, “Sensitized superbroadband near-IR emission in bismuth glass/Si nanocrystal superlattices,” Opt. Lett. 35(13), 2215–2217 (2010).
[Crossref] [PubMed]

H.-T. Sun, A. Hosokawa, Y. Miwa, F. Shimaoka, M. Fujii, M. Mizuhata, S. Hayashi, and S. Deki, “Strong ultra-broadband near-infrared photoluminescence from bismuth-embedded zeolites and their derivatives,” Adv. Mater. 21(36), 3694–3698 (2009).
[Crossref]

Tan, D.

Tan, D. Z.

B. B. Xu, S. F. Zhou, D. Z. Tan, Z. L. Hong, J. H. Hao, and J. R. Qiu, “Multifunctional tunable ultra-broadband visible and near-infrared luminescence from bismuth-doped germanate glasses,” J. Appl. Phys. 113(8), 083503 (2013).
[Crossref]

Tang, H.

Trusov, L. A.

A. A. Veber, A. N. Romanov, O. V. Usovich, Z. T. Fattakhova, E. V. Haula, V. N. Korchak, L. A. Trusov, P. E. Kazin, V. B. Sulimov, and V. B. Tsvetkov, “Luminescent properties of Bi-doped polycrystalline KAlCl4,” Appl. Phys. B 108(4), 733–736 (2012).
[Crossref]

Tsvetkov, V. B.

A. A. Veber, A. N. Romanov, O. V. Usovich, Z. T. Fattakhova, E. V. Haula, V. N. Korchak, L. A. Trusov, P. E. Kazin, V. B. Sulimov, and V. B. Tsvetkov, “Luminescent properties of Bi-doped polycrystalline KAlCl4,” Appl. Phys. B 108(4), 733–736 (2012).
[Crossref]

A. N. Romanov, E. V. Haula, Z. T. Fattakhova, A. A. Veber, V. B. Tsvetkov, D. M. Zhigunov, V. N. Korchak, and V. B. Sulimov, “Near-IR luminescence from subvalent bismuth species in fluoride glass,” Opt. Mater. 34(1), 155–158 (2011).
[Crossref]

Usovich, O. V.

A. A. Veber, A. N. Romanov, O. V. Usovich, Z. T. Fattakhova, E. V. Haula, V. N. Korchak, L. A. Trusov, P. E. Kazin, V. B. Sulimov, and V. B. Tsvetkov, “Luminescent properties of Bi-doped polycrystalline KAlCl4,” Appl. Phys. B 108(4), 733–736 (2012).
[Crossref]

Veber, A. A.

A. A. Veber, A. N. Romanov, O. V. Usovich, Z. T. Fattakhova, E. V. Haula, V. N. Korchak, L. A. Trusov, P. E. Kazin, V. B. Sulimov, and V. B. Tsvetkov, “Luminescent properties of Bi-doped polycrystalline KAlCl4,” Appl. Phys. B 108(4), 733–736 (2012).
[Crossref]

A. N. Romanov, E. V. Haula, Z. T. Fattakhova, A. A. Veber, V. B. Tsvetkov, D. M. Zhigunov, V. N. Korchak, and V. B. Sulimov, “Near-IR luminescence from subvalent bismuth species in fluoride glass,” Opt. Mater. 34(1), 155–158 (2011).
[Crossref]

Walsh, A.

L. Protesescu, S. Yakunin, M. I. Bodnarchuk, F. Krieg, R. Caputo, C. H. Hendon, R. X. Yang, A. Walsh, and M. V. Kovalenko, “Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut,” Nano Lett. 15(6), 3692–3696 (2015).
[Crossref] [PubMed]

Wang, L.

S. Gu, B. Zhou, W. Luo, L. Wang, W. Jiang, W. Jiang, and J. Ballato, “Near-infrared broadband photoluminescence of bismuth-doped zeolite-derived silica glass prepared by SPS,” J. Am. Ceram. Soc. 99(1), 121–127 (2016).
[Crossref]

Wang, R.

C. Li, Z. Song, J. Qiu, Z. Yang, X. Yu, D. Zhou, Z. Yin, R. Wang, Y. Xu, and Y. Cao, “Broadband yellow–white and near infrared luminescence from Bi-doped Ba10(PO4)6Cl2 prepared in reductive atmosphere,” J. Lumin. 132(7), 1807–1811 (2012).
[Crossref]

Wang, Y.

Y. Wang, X. Li, J. Song, L. Xiao, H. Zeng, and H. Sun, “All-Inorganic Colloidal Perovskite Quantum Dots: A New Class of Lasing Materials with Favorable Characteristics,” Adv. Mater. 27(44), 7101–7108 (2015).
[Crossref] [PubMed]

Wang, Z. W.

Y. Zhou, Z. J. Yong, K. C. Zhang, B. M. Liu, Z. W. Wang, J. S. Hou, Y. Z. Fang, Y. Zhou, H. T. Sun, and B. Song, “Ultrabroad Photoluminescence and Electroluminescence at New Wavelengths from Doped Organometal Halide Perovskites,” J. Phys. Chem. Lett. 7(14), 2735–2741 (2016).
[Crossref] [PubMed]

Wittmann, H. F.

J. C. de Mello, H. F. Wittmann, and R. H. Friend, “An Improved Experimental Determination of External Photoluminescence Quantum Efficiency,” Adv. Mater. 9(3), 230–232 (1997).
[Crossref]

Wu, F.

Wu, Y.

X. Li, Y. Wu, S. Zhang, B. Cai, Y. Gu, J. Song, and H. Zeng, “CsPbX3 Quantum Dots for Lighting and Displays: Room Temperature Synthesis, Photoluminescence Superiorities, Underlying Origins and White Light-Emitting Diodes,” Adv. Funct. Mater. 26(15), 2435–2445 (2016).
[Crossref]

Xia, H.

Xiao, L.

Y. Wang, X. Li, J. Song, L. Xiao, H. Zeng, and H. Sun, “All-Inorganic Colloidal Perovskite Quantum Dots: A New Class of Lasing Materials with Favorable Characteristics,” Adv. Mater. 27(44), 7101–7108 (2015).
[Crossref] [PubMed]

Xing, H.

Y. Zhou, D.-D. Zhou, B.-M. Liu, L.-N. Li, Z.-J. Yong, H. Xing, Y.-Z. Fang, J.-S. Hou, and H.-T. Sun, “Ultrabroad near-infrared photoluminescence from bismuth doped CsPbI3: polaronic defects vs. bismuth active centers,” J. Mater. Chem. C Mater. Opt. Electron. Devices 4(12), 2295–2301 (2016).
[Crossref]

Xu, B.

Xu, B. B.

B. B. Xu, S. F. Zhou, D. Z. Tan, Z. L. Hong, J. H. Hao, and J. R. Qiu, “Multifunctional tunable ultra-broadband visible and near-infrared luminescence from bismuth-doped germanate glasses,” J. Appl. Phys. 113(8), 083503 (2013).
[Crossref]

Xu, J.

Xu, Y.

C. Li, Z. Song, J. Qiu, Z. Yang, X. Yu, D. Zhou, Z. Yin, R. Wang, Y. Xu, and Y. Cao, “Broadband yellow–white and near infrared luminescence from Bi-doped Ba10(PO4)6Cl2 prepared in reductive atmosphere,” J. Lumin. 132(7), 1807–1811 (2012).
[Crossref]

Yakunin, S.

L. Protesescu, S. Yakunin, M. I. Bodnarchuk, F. Krieg, R. Caputo, C. H. Hendon, R. X. Yang, A. Walsh, and M. V. Kovalenko, “Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut,” Nano Lett. 15(6), 3692–3696 (2015).
[Crossref] [PubMed]

Yang, G.

B. M. Liu, Z. G. Zhang, K. Zhang, Y. Kuroiwa, C. Moriyoshi, H. M. Yu, C. Li, L. R. Zheng, L. N. Li, G. Yang, Y. Zhou, Y. Z. Fang, J. S. Hou, Y. Matsushita, and H. T. Sun, “Unconventional luminescent centers in metastable phases created by topochemical reduction reactions,” Angew. Chem. Int. Ed. Engl. 55(16), 4967–4971 (2016).
[Crossref] [PubMed]

Yang, J.

H. T. Sun, J. Yang, M. Fujii, Y. Sakka, Y. Zhu, T. Asahara, N. Shirahata, M. Ii, Z. Bai, J. G. Li, and H. Gao, “Highly fluorescent silica-coated bismuth-doped aluminosilicate nanoparticles for near-infrared bioimaging,” Small 7(2), 199–203 (2011).
[Crossref] [PubMed]

Yang, R. X.

L. Protesescu, S. Yakunin, M. I. Bodnarchuk, F. Krieg, R. Caputo, C. H. Hendon, R. X. Yang, A. Walsh, and M. V. Kovalenko, “Nanocrystals of Cesium Lead Halide Perovskites (CsPbX3, X = Cl, Br, and I): Novel Optoelectronic Materials Showing Bright Emission with Wide Color Gamut,” Nano Lett. 15(6), 3692–3696 (2015).
[Crossref] [PubMed]

Yang, Y.

Yang, Z.

C. Li, Z. Song, J. Qiu, Z. Yang, X. Yu, D. Zhou, Z. Yin, R. Wang, Y. Xu, and Y. Cao, “Broadband yellow–white and near infrared luminescence from Bi-doped Ba10(PO4)6Cl2 prepared in reductive atmosphere,” J. Lumin. 132(7), 1807–1811 (2012).
[Crossref]

Yin, Z.

C. Li, Z. Song, J. Qiu, Z. Yang, X. Yu, D. Zhou, Z. Yin, R. Wang, Y. Xu, and Y. Cao, “Broadband yellow–white and near infrared luminescence from Bi-doped Ba10(PO4)6Cl2 prepared in reductive atmosphere,” J. Lumin. 132(7), 1807–1811 (2012).
[Crossref]

Yong, Z. J.

Y. Zhou, Z. J. Yong, K. C. Zhang, B. M. Liu, Z. W. Wang, J. S. Hou, Y. Z. Fang, Y. Zhou, H. T. Sun, and B. Song, “Ultrabroad Photoluminescence and Electroluminescence at New Wavelengths from Doped Organometal Halide Perovskites,” J. Phys. Chem. Lett. 7(14), 2735–2741 (2016).
[Crossref] [PubMed]

Yong, Z.-J.

Y. Zhou, Z.-J. Yong, W. Zhang, J.-P. Ma, A. Sadhanala, Y.-M. Chen, B.-M. Liu, Y. Zhou, B. Song, and H.-T. Sun, “Ultra-broadband optical amplification at telecommunication wavelengths achieved by bismuth-activated lead iodide perovskites,” J. Mater. Chem. C Mater. Opt. Electron. Devices 5(10), 2591–2596 (2017).
[Crossref]

Y. Zhou, D.-D. Zhou, B.-M. Liu, L.-N. Li, Z.-J. Yong, H. Xing, Y.-Z. Fang, J.-S. Hou, and H.-T. Sun, “Ultrabroad near-infrared photoluminescence from bismuth doped CsPbI3: polaronic defects vs. bismuth active centers,” J. Mater. Chem. C Mater. Opt. Electron. Devices 4(12), 2295–2301 (2016).
[Crossref]

Yu, H. M.

B. M. Liu, Z. G. Zhang, K. Zhang, Y. Kuroiwa, C. Moriyoshi, H. M. Yu, C. Li, L. R. Zheng, L. N. Li, G. Yang, Y. Zhou, Y. Z. Fang, J. S. Hou, Y. Matsushita, and H. T. Sun, “Unconventional luminescent centers in metastable phases created by topochemical reduction reactions,” Angew. Chem. Int. Ed. Engl. 55(16), 4967–4971 (2016).
[Crossref] [PubMed]

Yu, J.

Yu, X.

C. Li, Z. Song, J. Qiu, Z. Yang, X. Yu, D. Zhou, Z. Yin, R. Wang, Y. Xu, and Y. Cao, “Broadband yellow–white and near infrared luminescence from Bi-doped Ba10(PO4)6Cl2 prepared in reductive atmosphere,” J. Lumin. 132(7), 1807–1811 (2012).
[Crossref]

Zagorodnev, V. N.

Zeng, H.

X. Li, Y. Wu, S. Zhang, B. Cai, Y. Gu, J. Song, and H. Zeng, “CsPbX3 Quantum Dots for Lighting and Displays: Room Temperature Synthesis, Photoluminescence Superiorities, Underlying Origins and White Light-Emitting Diodes,” Adv. Funct. Mater. 26(15), 2435–2445 (2016).
[Crossref]

Y. Wang, X. Li, J. Song, L. Xiao, H. Zeng, and H. Sun, “All-Inorganic Colloidal Perovskite Quantum Dots: A New Class of Lasing Materials with Favorable Characteristics,” Adv. Mater. 27(44), 7101–7108 (2015).
[Crossref] [PubMed]

Zhang, K.

B. M. Liu, Z. G. Zhang, K. Zhang, Y. Kuroiwa, C. Moriyoshi, H. M. Yu, C. Li, L. R. Zheng, L. N. Li, G. Yang, Y. Zhou, Y. Z. Fang, J. S. Hou, Y. Matsushita, and H. T. Sun, “Unconventional luminescent centers in metastable phases created by topochemical reduction reactions,” Angew. Chem. Int. Ed. Engl. 55(16), 4967–4971 (2016).
[Crossref] [PubMed]

Zhang, K. C.

Y. Zhou, Z. J. Yong, K. C. Zhang, B. M. Liu, Z. W. Wang, J. S. Hou, Y. Z. Fang, Y. Zhou, H. T. Sun, and B. Song, “Ultrabroad Photoluminescence and Electroluminescence at New Wavelengths from Doped Organometal Halide Perovskites,” J. Phys. Chem. Lett. 7(14), 2735–2741 (2016).
[Crossref] [PubMed]

Zhang, L.

Zhang, P.

Zhang, S.

X. Li, Y. Wu, S. Zhang, B. Cai, Y. Gu, J. Song, and H. Zeng, “CsPbX3 Quantum Dots for Lighting and Displays: Room Temperature Synthesis, Photoluminescence Superiorities, Underlying Origins and White Light-Emitting Diodes,” Adv. Funct. Mater. 26(15), 2435–2445 (2016).
[Crossref]

Zhang, W.

Y. Zhou, Z.-J. Yong, W. Zhang, J.-P. Ma, A. Sadhanala, Y.-M. Chen, B.-M. Liu, Y. Zhou, B. Song, and H.-T. Sun, “Ultra-broadband optical amplification at telecommunication wavelengths achieved by bismuth-activated lead iodide perovskites,” J. Mater. Chem. C Mater. Opt. Electron. Devices 5(10), 2591–2596 (2017).
[Crossref]

Zhang, X.

Zhang, Z. G.

B. M. Liu, Z. G. Zhang, K. Zhang, Y. Kuroiwa, C. Moriyoshi, H. M. Yu, C. Li, L. R. Zheng, L. N. Li, G. Yang, Y. Zhou, Y. Z. Fang, J. S. Hou, Y. Matsushita, and H. T. Sun, “Unconventional luminescent centers in metastable phases created by topochemical reduction reactions,” Angew. Chem. Int. Ed. Engl. 55(16), 4967–4971 (2016).
[Crossref] [PubMed]

Zhao, H.

Zheng, L.

Zheng, L. R.

B. M. Liu, Z. G. Zhang, K. Zhang, Y. Kuroiwa, C. Moriyoshi, H. M. Yu, C. Li, L. R. Zheng, L. N. Li, G. Yang, Y. Zhou, Y. Z. Fang, J. S. Hou, Y. Matsushita, and H. T. Sun, “Unconventional luminescent centers in metastable phases created by topochemical reduction reactions,” Angew. Chem. Int. Ed. Engl. 55(16), 4967–4971 (2016).
[Crossref] [PubMed]

Zhigunov, D. M.

A. N. Romanov, E. V. Haula, Z. T. Fattakhova, A. A. Veber, V. B. Tsvetkov, D. M. Zhigunov, V. N. Korchak, and V. B. Sulimov, “Near-IR luminescence from subvalent bismuth species in fluoride glass,” Opt. Mater. 34(1), 155–158 (2011).
[Crossref]

Zhou, B.

S. Gu, B. Zhou, W. Luo, L. Wang, W. Jiang, W. Jiang, and J. Ballato, “Near-infrared broadband photoluminescence of bismuth-doped zeolite-derived silica glass prepared by SPS,” J. Am. Ceram. Soc. 99(1), 121–127 (2016).
[Crossref]

Zhou, D.

C. Li, Z. Song, J. Qiu, Z. Yang, X. Yu, D. Zhou, Z. Yin, R. Wang, Y. Xu, and Y. Cao, “Broadband yellow–white and near infrared luminescence from Bi-doped Ba10(PO4)6Cl2 prepared in reductive atmosphere,” J. Lumin. 132(7), 1807–1811 (2012).
[Crossref]

Zhou, D.-D.

Y. Zhou, D.-D. Zhou, B.-M. Liu, L.-N. Li, Z.-J. Yong, H. Xing, Y.-Z. Fang, J.-S. Hou, and H.-T. Sun, “Ultrabroad near-infrared photoluminescence from bismuth doped CsPbI3: polaronic defects vs. bismuth active centers,” J. Mater. Chem. C Mater. Opt. Electron. Devices 4(12), 2295–2301 (2016).
[Crossref]

Zhou, J.

H.-T. Sun, J. Zhou, and J. Qiu, Prog. “Recent advances in bismuth activated photonic materials,” Prog. Mater. Sci. 64(10), 1–72 (2014).
[Crossref]

Zhou, P.

Zhou, S.

Zhou, S. F.

B. B. Xu, S. F. Zhou, D. Z. Tan, Z. L. Hong, J. H. Hao, and J. R. Qiu, “Multifunctional tunable ultra-broadband visible and near-infrared luminescence from bismuth-doped germanate glasses,” J. Appl. Phys. 113(8), 083503 (2013).
[Crossref]

Zhou, Y.

Y. Zhou, Z.-J. Yong, W. Zhang, J.-P. Ma, A. Sadhanala, Y.-M. Chen, B.-M. Liu, Y. Zhou, B. Song, and H.-T. Sun, “Ultra-broadband optical amplification at telecommunication wavelengths achieved by bismuth-activated lead iodide perovskites,” J. Mater. Chem. C Mater. Opt. Electron. Devices 5(10), 2591–2596 (2017).
[Crossref]

Y. Zhou, Z.-J. Yong, W. Zhang, J.-P. Ma, A. Sadhanala, Y.-M. Chen, B.-M. Liu, Y. Zhou, B. Song, and H.-T. Sun, “Ultra-broadband optical amplification at telecommunication wavelengths achieved by bismuth-activated lead iodide perovskites,” J. Mater. Chem. C Mater. Opt. Electron. Devices 5(10), 2591–2596 (2017).
[Crossref]

Y. Zhou, D.-D. Zhou, B.-M. Liu, L.-N. Li, Z.-J. Yong, H. Xing, Y.-Z. Fang, J.-S. Hou, and H.-T. Sun, “Ultrabroad near-infrared photoluminescence from bismuth doped CsPbI3: polaronic defects vs. bismuth active centers,” J. Mater. Chem. C Mater. Opt. Electron. Devices 4(12), 2295–2301 (2016).
[Crossref]

Y. Zhou, Z. J. Yong, K. C. Zhang, B. M. Liu, Z. W. Wang, J. S. Hou, Y. Z. Fang, Y. Zhou, H. T. Sun, and B. Song, “Ultrabroad Photoluminescence and Electroluminescence at New Wavelengths from Doped Organometal Halide Perovskites,” J. Phys. Chem. Lett. 7(14), 2735–2741 (2016).
[Crossref] [PubMed]

Y. Zhou, Z. J. Yong, K. C. Zhang, B. M. Liu, Z. W. Wang, J. S. Hou, Y. Z. Fang, Y. Zhou, H. T. Sun, and B. Song, “Ultrabroad Photoluminescence and Electroluminescence at New Wavelengths from Doped Organometal Halide Perovskites,” J. Phys. Chem. Lett. 7(14), 2735–2741 (2016).
[Crossref] [PubMed]

B. M. Liu, Z. G. Zhang, K. Zhang, Y. Kuroiwa, C. Moriyoshi, H. M. Yu, C. Li, L. R. Zheng, L. N. Li, G. Yang, Y. Zhou, Y. Z. Fang, J. S. Hou, Y. Matsushita, and H. T. Sun, “Unconventional luminescent centers in metastable phases created by topochemical reduction reactions,” Angew. Chem. Int. Ed. Engl. 55(16), 4967–4971 (2016).
[Crossref] [PubMed]

Zhu, Y.

H. T. Sun, J. Yang, M. Fujii, Y. Sakka, Y. Zhu, T. Asahara, N. Shirahata, M. Ii, Z. Bai, J. G. Li, and H. Gao, “Highly fluorescent silica-coated bismuth-doped aluminosilicate nanoparticles for near-infrared bioimaging,” Small 7(2), 199–203 (2011).
[Crossref] [PubMed]

Adv. Funct. Mater. (1)

X. Li, Y. Wu, S. Zhang, B. Cai, Y. Gu, J. Song, and H. Zeng, “CsPbX3 Quantum Dots for Lighting and Displays: Room Temperature Synthesis, Photoluminescence Superiorities, Underlying Origins and White Light-Emitting Diodes,” Adv. Funct. Mater. 26(15), 2435–2445 (2016).
[Crossref]

Adv. Mater. (3)

H.-T. Sun, A. Hosokawa, Y. Miwa, F. Shimaoka, M. Fujii, M. Mizuhata, S. Hayashi, and S. Deki, “Strong ultra-broadband near-infrared photoluminescence from bismuth-embedded zeolites and their derivatives,” Adv. Mater. 21(36), 3694–3698 (2009).
[Crossref]

J. C. de Mello, H. F. Wittmann, and R. H. Friend, “An Improved Experimental Determination of External Photoluminescence Quantum Efficiency,” Adv. Mater. 9(3), 230–232 (1997).
[Crossref]

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Opt. Express (3)

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Opt. Mater. (1)

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Small (1)

H. T. Sun, J. Yang, M. Fujii, Y. Sakka, Y. Zhu, T. Asahara, N. Shirahata, M. Ii, Z. Bai, J. G. Li, and H. Gao, “Highly fluorescent silica-coated bismuth-doped aluminosilicate nanoparticles for near-infrared bioimaging,” Small 7(2), 199–203 (2011).
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Figures (3)

Fig. 1
Fig. 1 Characterization of doped and undoped CsPbI3 NCs. (a) XRD patterns of undoped and Bi-doped CsPbI3 NCs with different Bi doping concentrations. The red vertical lines at the bottom correspond to the diffraction peaks of the cubic CsPbI3. TEM images and statistical distributions of the edge length of undoped (b/c) and 2%-doped (d/e) CsPbI3 NCs.
Fig. 2
Fig. 2 (a) Absorption and PL spectra of Bi doped and undoped CsPbI3 NCs. The PL spectra were obtained under 450 nm excitation. (b) Visible PL decay curves of Bi-doped and undoped CsPbI3 NCs.
Fig. 3
Fig. 3 (a) NIR PL excited by 450 nm and PLQY of Bi-doped CsPbI3 NCs with different nominal Bi concentrations. (b) NIR PL decays of Bi-doped CsPbI3 NCs. The monitored wavelength is 1145 nm. (c) Schematic illustration of the electronic transition in doped NCs. The thick and thin red lines represent the direct excitation of CsPbI3 NCs and nonradiative decay from the conduction band to the in-gap state, respectively. The violet line represents the NIR emission.

Equations (1)

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τ x = 0 t × I(t)dt 0 I(t)dt

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