Abstract

The nonlinear optical responses of two-dimensional (2D) few-layer tin diselenide (SnSe2) have been investigated in this work. By applying the Z-scan technique, the saturable absorption of SnSe2 thin film has been observed at a wavelength of ~1μm, which enables SnSe2, a new saturable absorber for pulsed laser generation. A detailed exploration of the nonlinear absorption of SnSe2 film and their dependence on excitation pulse energy is carried out. Our results show that saturation intensity of the nonlinear absorption is ~23.78 GW/cm2 and corresponding nonlinear absorption coefficients are at a range from −13596 to −2967.3 cm/GW. By employing the SnSe2-coated mirror as a saturable absorber, the passively Q-switched lasing has been achieved on a crystalline waveguide platform at ~1 μm.

© 2017 Optical Society of America

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2017 (2)

Z. T. Wang, H. R. Mu, J. Yuan, C. J. Zhao, Q. L. Bao, and H. Zhang, “Graphene-Bi2Te3 heterostructure as broadband saturable absorber for ultra-short pulse generation in Er-doped and Yb-doped fiber lasers,” IEEE J. Sel. Top. Quantum Electron. 23(1), 8800105 (2017).
[Crossref]

Y. Ding, B. Xiao, G. Tang, and J. Hong, “Transport Properties and High Thermopower of SnSe2: A Full Ab-Initio Investigation,” J. Phys. Chem. C 121(1), 225–236 (2017).
[Crossref]

2016 (14)

Y. Li, N. Dong, S. Zhang, K. Wang, L. Zhang, and J. Wang, “Optical identification of layered MoS2 via the characteristic matrix method,” Nanoscale 8(2), 1210–1215 (2016).
[Crossref] [PubMed]

Y. Tan, Z. Guo, L. Ma, H. Zhang, S. Akhmadaliev, S. Zhou, and F. Chen, “Q-switched waveguide laser based on two-dimensional semiconducting materials: tungsten disulfide and black phosphorous,” Opt. Express 24(3), 2858–2866 (2016).
[Crossref] [PubMed]

C. Cheng, H. Liu, Y. Tan, J. R. Vázquez de Aldana, and F. Chen, “Passively Q-switched waveguide lasers based on two-dimensional transition metal diselenide,” Opt. Express 24(10), 10385–10390 (2016).
[Crossref] [PubMed]

C. Cheng, H. L. Liu, Z. Shang, W. J. Nie, Y. Tan, B. R. Rabes, J. R. Vázquez de Aldana, D. Jaque, and F. Chen, “Femtosecond laser written waveguides with MoS2 as satuable absorber for passively Q-switched lasing,” Opt. Mater. Express 6(2), 367 (2016).
[Crossref]

Z. P. Sun, A. Martinez, and F. Wang, “Optical modulators with 2D layered materials,” Nat. Photonics 10(4), 227–238 (2016).
[Crossref]

W. J. Zhang, Q. X. Wang, Y. Chen, Z. Wang, and A. T. S. Wee, “Van der Waals stacked 2D layered materials for optoelectronics,” 2D. Mater. 3(2), 022001 (2016).
[Crossref]

J. P. Shi, Q. Q. Ji, Z. F. Liu, and Y. F. Zhang, “Recent Advances in Controlling Syntheses and Energy Related Applications of MX2 and MX2/Graphene Heterostructures,” Adv. Energy Mater. 6(17), 1600459 (2016).
[Crossref]

K. E. Aretouli, D. Tsoutsou, P. Tsipas, J. Marquez-Velasco, S. Aminalragia Giamini, N. Kelaidis, V. Psycharis, and A. Dimoulas, “Epitaxial 2D SnSe2/ 2D WSe2 van der Waals Heterostructures,” ACS Appl. Mater. Interfaces 8(35), 23222–23229 (2016).
[Crossref] [PubMed]

P. Yu, X. C. Yu, W. L. Lu, H. Lin, L. F. Sun, K. Z. Du, F. C. Liu, W. Fu, Q. S. Zeng, Z. X. Shen, C. H. Jin, Q. J. Wang, and Z. Liu, “Fast photoresponse from 1T Tin Diselenide atomic layers,” Adv. Funct. Mater. 26(1), 137–145 (2016).
[Crossref]

S. C. Dhanabalan, J. S. Ponraj, H. Zhang, and Q. Bao, “Present perspectives of broadband photodetectors based on nanobelts, nanoribbons, nanosheets and the emerging 2D materials,” Nanoscale 8(12), 6410–6434 (2016).
[Crossref] [PubMed]

J. M. Gonzalez and I. I. Oleynik, “Layer-dependent properties of SnS2 and SnSe2 two-dimensional materials,” Phys. Rev. B 94(12), 125443 (2016).
[Crossref]

Y. W. Wang, H. R. Mu, X. H. Li, J. Yuan, J. Z. Chen, S. Xiao, Q. L. Bao, Y. L. Gao, and J. He, “Observation of large nonlinear responses in a graphene-Bi2Te3 heterostructure at a telecommunication wavelength,” Appl. Phys. Lett. 108(22), 221901 (2016).
[Crossref]

F. Hipolito, T. G. Pedersen, and V. M. Pereira, “Nonlinear photocurrents in two-dimensional systems based on graphene and boron nitride,” Phys. Rev. B 94(4), 045434 (2016).
[Crossref]

K. Wang, B. M. Szydłowska, G. Wang, X. Zhang, J. J. Wang, J. J. Magan, L. Zhang, J. N. Coleman, J. Wang, and W. J. Blau, “Ultrafast nonlinear excitation dynamics of black phosphorus nanosheets from visible to mid-infrared,” ACS Nano 10(7), 6923–6932 (2016).
[Crossref] [PubMed]

2015 (7)

Z. N. Guo, H. Zhang, S. B. Lu, Z. T. Wang, S. Y. Tang, J. D. Shao, Z. B. Sun, H. H. Xie, H. Y. Wang, X. F. Yu, and P. K. Chu, “From black phosphorus to phosphorene: basic solvent exfoliation, evolution of raman scattering, and applications to ultrafast photonics,” Adv. Funct. Mater. 25(45), 6996–7002 (2015).
[Crossref]

S. B. Lu, L. L. Miao, Z. N. Guo, X. Qi, C. J. Zhao, H. Zhang, S. C. Wen, D. Y. Tang, and D. Y. Fan, “Broadband nonlinear optical response in multi-layer black phosphorus: an emerging infrared and mid-infrared optical material,” Opt. Express 23(9), 11183–11194 (2015).
[Crossref] [PubMed]

A. Gupta, T. Sakthivel, and S. Seal, “Recent development in 2D materials beyond graphene,” Prog. Mater. Sci. 73, 44–126 (2015).
[Crossref]

A. Taube, A. Łapinska, J. Judek, and M. Zdrojekc, “Temperature dependence of Raman shifts in layered ReSe2 and SnSe2 semiconductor nanosheets,” Appl. Phys. Lett. 107(1), 013105 (2015).
[Crossref]

N. Dong, Y. Li, Y. Feng, S. Zhang, X. Zhang, C. Chang, J. Fan, L. Zhang, and J. Wang, “Optical limiting and theoretical modelling of layered transition metal dichalcogenide nanosheets,” Sci. Rep. 5, 14646 (2015).
[Crossref] [PubMed]

S. Zhang, N. Dong, N. McEvoy, M. O’Brien, S. Winters, N. C. Berner, C. Yim, Y. Li, X. Zhang, Z. Chen, L. Zhang, G. S. Duesberg, and J. Wang, “Direct observation of degenerate two-photon absorption and its saturation in WS2 and MoS2 monolayer and few-layer films,” ACS Nano 9(7), 7142–7150 (2015).
[Crossref] [PubMed]

X. Zhou, L. Gan, W. Tian, Q. Zhang, S. Jin, H. Li, Y. Bando, D. Golberg, and T. Zhai, “Ultrathin SnSe2 flakes grown by chemical vapor deposition for high-performance photodetectors,” Adv. Mater. 27(48), 8035–8041 (2015).
[Crossref] [PubMed]

2014 (4)

J. Du, Q. Wang, G. Jiang, C. Xu, C. Zhao, Y. Xiang, Y. Chen, S. Wen, and H. Zhang, “Ytterbium-doped fiber laser passively mode locked by few-layer Molybdenum Disulfide (MoS2) saturable absorber functioned with evanescent field interaction,” Sci. Rep. 4, 6346 (2014).
[Crossref] [PubMed]

D. Jariwala, V. K. Sangwan, L. J. Lauhon, T. J. Marks, and M. C. Hersam, “Emerging device applications for semiconducting two-dimensional transition metal dichalcogenides,” ACS Nano 8(2), 1102–1120 (2014).
[Crossref] [PubMed]

C. Zhang, H. Yin, M. Han, Z. Dai, H. Pang, Y. Zheng, Y. Q. Lan, J. Bao, and J. Zhu, “Two-dimensional tin selenide nanostructures for flexible all-solid-state supercapacitors,” ACS Nano 8(4), 3761–3770 (2014).
[Crossref] [PubMed]

C. Y. Ling, Y. C. Huang, H. Liu, S. F. Wang, Z. Fang, and L. X. Ning, “Mechanical properties, electronic structures, and potential applications in lithium ion batteries: a first-principles study toward SnSe2 nanotubes,” J. Phys. Chem. C 118(48), 28291–28298 (2014).
[Crossref]

2013 (2)

S. Z. Butler, S. M. Hollen, L. Cao, Y. Cui, J. A. Gupta, H. R. Gutiérrez, T. F. Heinz, S. S. Hong, J. Huang, A. F. Ismach, E. Johnston-Halperin, M. Kuno, V. V. Plashnitsa, R. D. Robinson, R. S. Ruoff, S. Salahuddin, J. Shan, L. Shi, M. G. Spencer, M. Terrones, W. Windl, and J. E. Goldberger, “Progress, challenges, and opportunities in two-dimensional materials beyond graphene,” ACS Nano 7(4), 2898–2926 (2013).
[Crossref] [PubMed]

K. Wang, J. Wang, J. Fan, M. Lotya, A. O’Neill, D. Fox, Y. Feng, X. Zhang, B. Jiang, Q. Zhao, H. Zhang, J. N. Coleman, L. Zhang, and W. J. Blau, “Ultrafast saturable absorption of two-dimensional MoS2 nanosheets,” ACS Nano 7(10), 9260–9267 (2013).
[Crossref] [PubMed]

2012 (2)

Q. H. Wang, K. Kalantar-Zadeh, A. Kis, J. N. Coleman, and M. S. Strano, “Electronics and optoelectronics of two-dimensional transition metal dichalcogenides,” Nat. Nanotechnol. 7(11), 699–712 (2012).
[Crossref] [PubMed]

X. Yu, J. Zhu, Y. Zhang, J. Weng, L. Hu, and S. Dai, “SnSe2 quantum dot sensitized solar cells prepared employing molecular metal chalcogenide as precursors,” Chem. Commun. (Camb.) 48(27), 3324–3326 (2012).
[Crossref] [PubMed]

2011 (1)

R. Y. Wang, M. A. Caldwell, R. G. D. Jeyasingh, S. Aloni, R. M. Shelby, H.-S. P. Wong, and D. J. Milliron, “Electronic and optical switching of solution-phase deposited SnSe2 phase change memory material,” J. Appl. Phys. 109(11), 113506 (2011).
[Crossref]

2010 (1)

F. Bonaccorso, Z. Sun, T. Hasan, and A. C. Ferrari, “Graphene photonics and optoelectronics,” Nat. Photonics 4(9), 611–622 (2010).
[Crossref]

2007 (1)

A. K. Geim and K. S. Novoselov, “The rise of graphene,” Nat. Mater. 6(3), 183–191 (2007).
[Crossref] [PubMed]

2004 (1)

K. S. Novoselov, A. K. Geim, S. V. Morozov, D. Jiang, Y. Zhang, S. V. Dubonos, I. V. Grigorieva, and A. A. Firsov, “Electric field effect in atomically thin carbon films,” Science 306(5696), 666–669 (2004).
[Crossref] [PubMed]

1996 (2)

L. C. Oliveira, T. Catunda, and C. Zilio, “Saturation effects in Z-scan measurements,” Jpn. J. Appl. Phys. 35(5A), 2649–2652 (1996).
[Crossref]

U. Keller, K. J. Weingarten, F. X. Kartner, D. Kopf, B. Braun, I. D. Jung, and J. A. Der Au, “Semiconductor saturable absorber mirrors (SESAM’s) for femtosecond to nanosecond pulse generation in solid-state lasers,” IEEE J. Sel. Top. Quantum Electron. 2(3), 435–453 (1996).
[Crossref]

Akhmadaliev, S.

Aloni, S.

R. Y. Wang, M. A. Caldwell, R. G. D. Jeyasingh, S. Aloni, R. M. Shelby, H.-S. P. Wong, and D. J. Milliron, “Electronic and optical switching of solution-phase deposited SnSe2 phase change memory material,” J. Appl. Phys. 109(11), 113506 (2011).
[Crossref]

Aminalragia Giamini, S.

K. E. Aretouli, D. Tsoutsou, P. Tsipas, J. Marquez-Velasco, S. Aminalragia Giamini, N. Kelaidis, V. Psycharis, and A. Dimoulas, “Epitaxial 2D SnSe2/ 2D WSe2 van der Waals Heterostructures,” ACS Appl. Mater. Interfaces 8(35), 23222–23229 (2016).
[Crossref] [PubMed]

Aretouli, K. E.

K. E. Aretouli, D. Tsoutsou, P. Tsipas, J. Marquez-Velasco, S. Aminalragia Giamini, N. Kelaidis, V. Psycharis, and A. Dimoulas, “Epitaxial 2D SnSe2/ 2D WSe2 van der Waals Heterostructures,” ACS Appl. Mater. Interfaces 8(35), 23222–23229 (2016).
[Crossref] [PubMed]

Bando, Y.

X. Zhou, L. Gan, W. Tian, Q. Zhang, S. Jin, H. Li, Y. Bando, D. Golberg, and T. Zhai, “Ultrathin SnSe2 flakes grown by chemical vapor deposition for high-performance photodetectors,” Adv. Mater. 27(48), 8035–8041 (2015).
[Crossref] [PubMed]

Bao, J.

C. Zhang, H. Yin, M. Han, Z. Dai, H. Pang, Y. Zheng, Y. Q. Lan, J. Bao, and J. Zhu, “Two-dimensional tin selenide nanostructures for flexible all-solid-state supercapacitors,” ACS Nano 8(4), 3761–3770 (2014).
[Crossref] [PubMed]

Bao, Q.

S. C. Dhanabalan, J. S. Ponraj, H. Zhang, and Q. Bao, “Present perspectives of broadband photodetectors based on nanobelts, nanoribbons, nanosheets and the emerging 2D materials,” Nanoscale 8(12), 6410–6434 (2016).
[Crossref] [PubMed]

Bao, Q. L.

Z. T. Wang, H. R. Mu, J. Yuan, C. J. Zhao, Q. L. Bao, and H. Zhang, “Graphene-Bi2Te3 heterostructure as broadband saturable absorber for ultra-short pulse generation in Er-doped and Yb-doped fiber lasers,” IEEE J. Sel. Top. Quantum Electron. 23(1), 8800105 (2017).
[Crossref]

Y. W. Wang, H. R. Mu, X. H. Li, J. Yuan, J. Z. Chen, S. Xiao, Q. L. Bao, Y. L. Gao, and J. He, “Observation of large nonlinear responses in a graphene-Bi2Te3 heterostructure at a telecommunication wavelength,” Appl. Phys. Lett. 108(22), 221901 (2016).
[Crossref]

Berner, N. C.

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Tang, G.

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Y. Li, N. Dong, S. Zhang, K. Wang, L. Zhang, and J. Wang, “Optical identification of layered MoS2 via the characteristic matrix method,” Nanoscale 8(2), 1210–1215 (2016).
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W. J. Zhang, Q. X. Wang, Y. Chen, Z. Wang, and A. T. S. Wee, “Van der Waals stacked 2D layered materials for optoelectronics,” 2D. Mater. 3(2), 022001 (2016).
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Z. T. Wang, H. R. Mu, J. Yuan, C. J. Zhao, Q. L. Bao, and H. Zhang, “Graphene-Bi2Te3 heterostructure as broadband saturable absorber for ultra-short pulse generation in Er-doped and Yb-doped fiber lasers,” IEEE J. Sel. Top. Quantum Electron. 23(1), 8800105 (2017).
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Z. N. Guo, H. Zhang, S. B. Lu, Z. T. Wang, S. Y. Tang, J. D. Shao, Z. B. Sun, H. H. Xie, H. Y. Wang, X. F. Yu, and P. K. Chu, “From black phosphorus to phosphorene: basic solvent exfoliation, evolution of raman scattering, and applications to ultrafast photonics,” Adv. Funct. Mater. 25(45), 6996–7002 (2015).
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Weng, J.

X. Yu, J. Zhu, Y. Zhang, J. Weng, L. Hu, and S. Dai, “SnSe2 quantum dot sensitized solar cells prepared employing molecular metal chalcogenide as precursors,” Chem. Commun. (Camb.) 48(27), 3324–3326 (2012).
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S. Z. Butler, S. M. Hollen, L. Cao, Y. Cui, J. A. Gupta, H. R. Gutiérrez, T. F. Heinz, S. S. Hong, J. Huang, A. F. Ismach, E. Johnston-Halperin, M. Kuno, V. V. Plashnitsa, R. D. Robinson, R. S. Ruoff, S. Salahuddin, J. Shan, L. Shi, M. G. Spencer, M. Terrones, W. Windl, and J. E. Goldberger, “Progress, challenges, and opportunities in two-dimensional materials beyond graphene,” ACS Nano 7(4), 2898–2926 (2013).
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S. Zhang, N. Dong, N. McEvoy, M. O’Brien, S. Winters, N. C. Berner, C. Yim, Y. Li, X. Zhang, Z. Chen, L. Zhang, G. S. Duesberg, and J. Wang, “Direct observation of degenerate two-photon absorption and its saturation in WS2 and MoS2 monolayer and few-layer films,” ACS Nano 9(7), 7142–7150 (2015).
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J. Du, Q. Wang, G. Jiang, C. Xu, C. Zhao, Y. Xiang, Y. Chen, S. Wen, and H. Zhang, “Ytterbium-doped fiber laser passively mode locked by few-layer Molybdenum Disulfide (MoS2) saturable absorber functioned with evanescent field interaction,” Sci. Rep. 4, 6346 (2014).
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Y. Ding, B. Xiao, G. Tang, and J. Hong, “Transport Properties and High Thermopower of SnSe2: A Full Ab-Initio Investigation,” J. Phys. Chem. C 121(1), 225–236 (2017).
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Y. W. Wang, H. R. Mu, X. H. Li, J. Yuan, J. Z. Chen, S. Xiao, Q. L. Bao, Y. L. Gao, and J. He, “Observation of large nonlinear responses in a graphene-Bi2Te3 heterostructure at a telecommunication wavelength,” Appl. Phys. Lett. 108(22), 221901 (2016).
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Z. N. Guo, H. Zhang, S. B. Lu, Z. T. Wang, S. Y. Tang, J. D. Shao, Z. B. Sun, H. H. Xie, H. Y. Wang, X. F. Yu, and P. K. Chu, “From black phosphorus to phosphorene: basic solvent exfoliation, evolution of raman scattering, and applications to ultrafast photonics,” Adv. Funct. Mater. 25(45), 6996–7002 (2015).
[Crossref]

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J. Du, Q. Wang, G. Jiang, C. Xu, C. Zhao, Y. Xiang, Y. Chen, S. Wen, and H. Zhang, “Ytterbium-doped fiber laser passively mode locked by few-layer Molybdenum Disulfide (MoS2) saturable absorber functioned with evanescent field interaction,” Sci. Rep. 4, 6346 (2014).
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Yim, C.

S. Zhang, N. Dong, N. McEvoy, M. O’Brien, S. Winters, N. C. Berner, C. Yim, Y. Li, X. Zhang, Z. Chen, L. Zhang, G. S. Duesberg, and J. Wang, “Direct observation of degenerate two-photon absorption and its saturation in WS2 and MoS2 monolayer and few-layer films,” ACS Nano 9(7), 7142–7150 (2015).
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C. Zhang, H. Yin, M. Han, Z. Dai, H. Pang, Y. Zheng, Y. Q. Lan, J. Bao, and J. Zhu, “Two-dimensional tin selenide nanostructures for flexible all-solid-state supercapacitors,” ACS Nano 8(4), 3761–3770 (2014).
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[Crossref]

Yu, X.

X. Yu, J. Zhu, Y. Zhang, J. Weng, L. Hu, and S. Dai, “SnSe2 quantum dot sensitized solar cells prepared employing molecular metal chalcogenide as precursors,” Chem. Commun. (Camb.) 48(27), 3324–3326 (2012).
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P. Yu, X. C. Yu, W. L. Lu, H. Lin, L. F. Sun, K. Z. Du, F. C. Liu, W. Fu, Q. S. Zeng, Z. X. Shen, C. H. Jin, Q. J. Wang, and Z. Liu, “Fast photoresponse from 1T Tin Diselenide atomic layers,” Adv. Funct. Mater. 26(1), 137–145 (2016).
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Z. N. Guo, H. Zhang, S. B. Lu, Z. T. Wang, S. Y. Tang, J. D. Shao, Z. B. Sun, H. H. Xie, H. Y. Wang, X. F. Yu, and P. K. Chu, “From black phosphorus to phosphorene: basic solvent exfoliation, evolution of raman scattering, and applications to ultrafast photonics,” Adv. Funct. Mater. 25(45), 6996–7002 (2015).
[Crossref]

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Z. T. Wang, H. R. Mu, J. Yuan, C. J. Zhao, Q. L. Bao, and H. Zhang, “Graphene-Bi2Te3 heterostructure as broadband saturable absorber for ultra-short pulse generation in Er-doped and Yb-doped fiber lasers,” IEEE J. Sel. Top. Quantum Electron. 23(1), 8800105 (2017).
[Crossref]

Y. W. Wang, H. R. Mu, X. H. Li, J. Yuan, J. Z. Chen, S. Xiao, Q. L. Bao, Y. L. Gao, and J. He, “Observation of large nonlinear responses in a graphene-Bi2Te3 heterostructure at a telecommunication wavelength,” Appl. Phys. Lett. 108(22), 221901 (2016).
[Crossref]

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A. Taube, A. Łapinska, J. Judek, and M. Zdrojekc, “Temperature dependence of Raman shifts in layered ReSe2 and SnSe2 semiconductor nanosheets,” Appl. Phys. Lett. 107(1), 013105 (2015).
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P. Yu, X. C. Yu, W. L. Lu, H. Lin, L. F. Sun, K. Z. Du, F. C. Liu, W. Fu, Q. S. Zeng, Z. X. Shen, C. H. Jin, Q. J. Wang, and Z. Liu, “Fast photoresponse from 1T Tin Diselenide atomic layers,” Adv. Funct. Mater. 26(1), 137–145 (2016).
[Crossref]

Zhai, T.

X. Zhou, L. Gan, W. Tian, Q. Zhang, S. Jin, H. Li, Y. Bando, D. Golberg, and T. Zhai, “Ultrathin SnSe2 flakes grown by chemical vapor deposition for high-performance photodetectors,” Adv. Mater. 27(48), 8035–8041 (2015).
[Crossref] [PubMed]

Zhang, C.

C. Zhang, H. Yin, M. Han, Z. Dai, H. Pang, Y. Zheng, Y. Q. Lan, J. Bao, and J. Zhu, “Two-dimensional tin selenide nanostructures for flexible all-solid-state supercapacitors,” ACS Nano 8(4), 3761–3770 (2014).
[Crossref] [PubMed]

Zhang, H.

Z. T. Wang, H. R. Mu, J. Yuan, C. J. Zhao, Q. L. Bao, and H. Zhang, “Graphene-Bi2Te3 heterostructure as broadband saturable absorber for ultra-short pulse generation in Er-doped and Yb-doped fiber lasers,” IEEE J. Sel. Top. Quantum Electron. 23(1), 8800105 (2017).
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S. B. Lu, L. L. Miao, Z. N. Guo, X. Qi, C. J. Zhao, H. Zhang, S. C. Wen, D. Y. Tang, and D. Y. Fan, “Broadband nonlinear optical response in multi-layer black phosphorus: an emerging infrared and mid-infrared optical material,” Opt. Express 23(9), 11183–11194 (2015).
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J. Du, Q. Wang, G. Jiang, C. Xu, C. Zhao, Y. Xiang, Y. Chen, S. Wen, and H. Zhang, “Ytterbium-doped fiber laser passively mode locked by few-layer Molybdenum Disulfide (MoS2) saturable absorber functioned with evanescent field interaction,” Sci. Rep. 4, 6346 (2014).
[Crossref] [PubMed]

K. Wang, J. Wang, J. Fan, M. Lotya, A. O’Neill, D. Fox, Y. Feng, X. Zhang, B. Jiang, Q. Zhao, H. Zhang, J. N. Coleman, L. Zhang, and W. J. Blau, “Ultrafast saturable absorption of two-dimensional MoS2 nanosheets,” ACS Nano 7(10), 9260–9267 (2013).
[Crossref] [PubMed]

Zhang, L.

Y. Li, N. Dong, S. Zhang, K. Wang, L. Zhang, and J. Wang, “Optical identification of layered MoS2 via the characteristic matrix method,” Nanoscale 8(2), 1210–1215 (2016).
[Crossref] [PubMed]

K. Wang, B. M. Szydłowska, G. Wang, X. Zhang, J. J. Wang, J. J. Magan, L. Zhang, J. N. Coleman, J. Wang, and W. J. Blau, “Ultrafast nonlinear excitation dynamics of black phosphorus nanosheets from visible to mid-infrared,” ACS Nano 10(7), 6923–6932 (2016).
[Crossref] [PubMed]

N. Dong, Y. Li, Y. Feng, S. Zhang, X. Zhang, C. Chang, J. Fan, L. Zhang, and J. Wang, “Optical limiting and theoretical modelling of layered transition metal dichalcogenide nanosheets,” Sci. Rep. 5, 14646 (2015).
[Crossref] [PubMed]

S. Zhang, N. Dong, N. McEvoy, M. O’Brien, S. Winters, N. C. Berner, C. Yim, Y. Li, X. Zhang, Z. Chen, L. Zhang, G. S. Duesberg, and J. Wang, “Direct observation of degenerate two-photon absorption and its saturation in WS2 and MoS2 monolayer and few-layer films,” ACS Nano 9(7), 7142–7150 (2015).
[Crossref] [PubMed]

K. Wang, J. Wang, J. Fan, M. Lotya, A. O’Neill, D. Fox, Y. Feng, X. Zhang, B. Jiang, Q. Zhao, H. Zhang, J. N. Coleman, L. Zhang, and W. J. Blau, “Ultrafast saturable absorption of two-dimensional MoS2 nanosheets,” ACS Nano 7(10), 9260–9267 (2013).
[Crossref] [PubMed]

Zhang, Q.

X. Zhou, L. Gan, W. Tian, Q. Zhang, S. Jin, H. Li, Y. Bando, D. Golberg, and T. Zhai, “Ultrathin SnSe2 flakes grown by chemical vapor deposition for high-performance photodetectors,” Adv. Mater. 27(48), 8035–8041 (2015).
[Crossref] [PubMed]

Zhang, S.

Y. Li, N. Dong, S. Zhang, K. Wang, L. Zhang, and J. Wang, “Optical identification of layered MoS2 via the characteristic matrix method,” Nanoscale 8(2), 1210–1215 (2016).
[Crossref] [PubMed]

N. Dong, Y. Li, Y. Feng, S. Zhang, X. Zhang, C. Chang, J. Fan, L. Zhang, and J. Wang, “Optical limiting and theoretical modelling of layered transition metal dichalcogenide nanosheets,” Sci. Rep. 5, 14646 (2015).
[Crossref] [PubMed]

S. Zhang, N. Dong, N. McEvoy, M. O’Brien, S. Winters, N. C. Berner, C. Yim, Y. Li, X. Zhang, Z. Chen, L. Zhang, G. S. Duesberg, and J. Wang, “Direct observation of degenerate two-photon absorption and its saturation in WS2 and MoS2 monolayer and few-layer films,” ACS Nano 9(7), 7142–7150 (2015).
[Crossref] [PubMed]

Zhang, W. J.

W. J. Zhang, Q. X. Wang, Y. Chen, Z. Wang, and A. T. S. Wee, “Van der Waals stacked 2D layered materials for optoelectronics,” 2D. Mater. 3(2), 022001 (2016).
[Crossref]

Zhang, X.

K. Wang, B. M. Szydłowska, G. Wang, X. Zhang, J. J. Wang, J. J. Magan, L. Zhang, J. N. Coleman, J. Wang, and W. J. Blau, “Ultrafast nonlinear excitation dynamics of black phosphorus nanosheets from visible to mid-infrared,” ACS Nano 10(7), 6923–6932 (2016).
[Crossref] [PubMed]

S. Zhang, N. Dong, N. McEvoy, M. O’Brien, S. Winters, N. C. Berner, C. Yim, Y. Li, X. Zhang, Z. Chen, L. Zhang, G. S. Duesberg, and J. Wang, “Direct observation of degenerate two-photon absorption and its saturation in WS2 and MoS2 monolayer and few-layer films,” ACS Nano 9(7), 7142–7150 (2015).
[Crossref] [PubMed]

N. Dong, Y. Li, Y. Feng, S. Zhang, X. Zhang, C. Chang, J. Fan, L. Zhang, and J. Wang, “Optical limiting and theoretical modelling of layered transition metal dichalcogenide nanosheets,” Sci. Rep. 5, 14646 (2015).
[Crossref] [PubMed]

K. Wang, J. Wang, J. Fan, M. Lotya, A. O’Neill, D. Fox, Y. Feng, X. Zhang, B. Jiang, Q. Zhao, H. Zhang, J. N. Coleman, L. Zhang, and W. J. Blau, “Ultrafast saturable absorption of two-dimensional MoS2 nanosheets,” ACS Nano 7(10), 9260–9267 (2013).
[Crossref] [PubMed]

Zhang, Y.

X. Yu, J. Zhu, Y. Zhang, J. Weng, L. Hu, and S. Dai, “SnSe2 quantum dot sensitized solar cells prepared employing molecular metal chalcogenide as precursors,” Chem. Commun. (Camb.) 48(27), 3324–3326 (2012).
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K. S. Novoselov, A. K. Geim, S. V. Morozov, D. Jiang, Y. Zhang, S. V. Dubonos, I. V. Grigorieva, and A. A. Firsov, “Electric field effect in atomically thin carbon films,” Science 306(5696), 666–669 (2004).
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Zhang, Y. F.

J. P. Shi, Q. Q. Ji, Z. F. Liu, and Y. F. Zhang, “Recent Advances in Controlling Syntheses and Energy Related Applications of MX2 and MX2/Graphene Heterostructures,” Adv. Energy Mater. 6(17), 1600459 (2016).
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Zhao, C.

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Figures (8)

Fig. 1
Fig. 1 (a) AFM image of SnSe2 thin film and measurement of height, (b) linear absorption as functions of wavelength and photon energy, corresponding to top and bottom axes.
Fig. 2
Fig. 2 (a) Schematic of in- and out-plane Raman modes, (b) measured Raman spectrum.
Fig. 3
Fig. 3 The schematic of the experimental setup of the Z-scan system in this work.
Fig. 4
Fig. 4 non-linear absorbance detected by the Z-scan system.
Fig. 5
Fig. 5 Fitting values of nonlinear coefficient β as functions of the different excitation irradiance, and their fitted curves.
Fig. 6
Fig. 6 Schematic of the experimental setup for the Q-switched waveguide laser generation; the insert is the SA of SnSe2.
Fig. 7
Fig. 7 The average output power as a function of incident power (a), emission spectrum of Q-switched waveguide laser system (b), and the pulse trains output at (c) TE- and (d) TM-polarized light pump.
Fig. 8
Fig. 8 The Q-switched waveguide laser (a) parameters of repetition rates and pulse durations, and (b) values of pulse energy and peak power, in TE- and TM-polarization.

Tables (1)

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Table 1 Comparison of Q-switched Waveguide Lasers Based on Different 2D Materials

Equations (4)

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d I d z = α ( I ) I
α ( I ) = α 0 + β I
α ( I ) = α 0 1 + I / I S
E p h ν L σ L V q η o u t

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