Abstract

Optically active perovskite nanocrystals have shown considerable promise for a myriad of applications, such as single photon source, light-emitting diodes and nanophotonics. Coupling those nanocrystals to photonic micro- and nanostructures will offer additional degrees of freedom to manipulate their optical properties. Herein, we demonstrate the coupling of perovskite nanocrystals to a mechanically robust, poly(methyl-methacrylate) (PMMA)-encapsulated silicon nitride nanobeam photonic crystal cavity at room temperature. As determined from the time-resolved photoluminescence decay measurements, we observed enhanced spontaneous emission from the perovskite nanocrystals by a factor of 1.4, consistent with finite difference time domain simulation. In addition, by varying the concentration of the perovskite nanocrystal in the PMMA layer, the effective index of the layer can be modified, allowing us to tune the cavity mode resonance. Our results show that solution-processable perovskite nanocrystals hold a promising prospect for applications such as on-chip light sources, optoelectronic devices and photonic integrated circuits.

© 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

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2019 (1)

Y. Fu, H. Zhu, J. Chen, M. P. Hautzinger, X.-Y. Zhu, and S. Jin, “Metal halide perovskite nanostructures for optoelectronic applications and the study of physical properties,” Nat. Rev. Mater. 4(3), 169–188 (2019).
[Crossref]

2018 (7)

K. Lin, J. Xing, L. N. Quan, F. P. G. de Arquer, X. Gong, J. Lu, L. Xie, W. Zhao, D. Zhang, C. Yan, W. Li, X. Liu, Y. Lu, J. Kirman, E. H. Sargent, Q. Xiong, and Z. Wei, “Perovskite light-emitting diodes with external quantum efficiency exceeding 20 per cent,” Nature 562(7726), 245–248 (2018).
[Crossref] [PubMed]

K. Wang, S. Wang, S. Xiao, and Q. Song, “Recent advances in perovskite micro- and nanolasers,” Adv. Opt. Mater. 6(18), 1800278 (2018).
[Crossref]

F. Yan, J. Xing, G. Xing, L. Quan, S. T. Tan, J. Zhao, R. Su, L. Zhang, S. Chen, Y. Zhao, A. Huan, E. H. Sargent, Q. Xiong, and H. V. Demir, “Highly Efficient Visible Colloidal Lead-Halide Perovskite Nanocrystal Light-Emitting Diodes,” Nano Lett. 18(5), 3157–3164 (2018).
[Crossref] [PubMed]

S. Ma, M. Cai, T. Cheng, X. Ding, X. Shi, A. Alsaedi, T. Hayat, Y. Ding, Z. Tan, and S. Dai, “Two-dimensional organic-inorganic hybrid perovskite: from material properties to device applications,” Sci. China Mater. 61(10), 1257–1277 (2018).
[Crossref]

T. K. Fryett, Y. Chen, J. Whitehead, Z. M. Peycke, X. Xu, and A. Majumdar, “Encapsulated silicon nitride nanobeam cavity for hybrid nanophotonics,” ACS Photonics 5(6), 2176–2181 (2018).
[Crossref]

Y. Chen, A. Ryou, M. R. Friedfeld, T. Fryett, J. Whitehead, B. M. Cossairt, and A. Majumdar, “Deterministic positioning of colloidal quantum dots on silicon nitride nanobeam cavities,” Nano Lett. 18(10), 6404–6410 (2018).
[Crossref] [PubMed]

M. A. Becker, R. Vaxenburg, G. Nedelcu, P. C. Sercel, A. Shabaev, M. J. Mehl, J. G. Michopoulos, S. G. Lambrakos, N. Bernstein, J. L. Lyons, T. Stöferle, R. F. Mahrt, M. V. Kovalenko, D. J. Norris, G. Rainò, and A. L. Efros, “Bright triplet excitons in caesium lead halide perovskites,” Nature 553(7687), 189–193 (2018).
[Crossref] [PubMed]

2017 (10)

B. Cai, X. Li, Y. Gu, M. Harb, J. Li, M. Xie, F. Cao, J. Song, S. Zhang, L. Cavallo, and H. Zeng, “Quantum confinement effect of two-dimensional all-inorganic halide perovskites,” Sci. China Mater. 60(9), 811–818 (2017).
[Crossref]

Z. Yang, M. Pelton, M. I. Bodnarchuk, M. V. Kovalenko, and E. Waks, “Spontaneous emission enhancement of colloidal perovskite nanocrystals by a photonic crystal cavity,” Appl. Phys. Lett. 111(22), 221104 (2017).
[Crossref]

S. Schünemann, S. Brittman, K. Chen, E. C. Garnett, and H. Tüysüz, “Halide perovskite 3D photonic crystals for distributed feedback lasers,” ACS Photonics 4(10), 2522–2528 (2017).
[Crossref]

J. Wu, J. Chen, Y. Zhang, Z. Xu, L. Zhao, T. Liu, D. Luo, W. Yang, K. Chen, Q. Hu, F. Ye, P. Wu, R. Zhu, and Q. Gong, “Pinhole-free hybrid perovskite film with arbitrarily-shaped micro-patterns for functional optoelectronic devices,” Nano Lett. 17(6), 3563–3569 (2017).
[Crossref] [PubMed]

R. Su, C. Diederichs, J. Wang, T. C. H. Liew, J. Zhao, S. Liu, W. Xu, Z. Chen, and Q. Xiong, “Room-temperature polariton lasing in all-inorganic perovskite nanoplatelets,” Nano Lett. 17(6), 3982–3988 (2017).
[Crossref] [PubMed]

Q. Zhang, R. Su, W. Du, X. Liu, L. Zhao, S. T. Ha, and Q. Xiong, “Advances in Small Perovskite-Based Lasers,” Small Methods 1(9), 1700163 (2017).
[Crossref]

T. Thu Ha Do, A. Granados del Águila, C. Cui, J. Xing, Z. Ning, and Q. Xiong, “Optical study on intrinsic exciton states in high-quality CH3NH3PbBr3 single crystals,” Phys. Rev. B 96(7), 075308 (2017).
[Crossref]

C. Yin, L. Chen, N. Song, Y. Lv, F. Hu, C. Sun, W. W. Yu, C. Zhang, X. Wang, Y. Zhang, and M. Xiao, “Bright-exciton fine-structure splittings in single perovskite nanocrystals,” Phys. Rev. Lett. 119(2), 026401 (2017).
[Crossref] [PubMed]

S.-T. Ha, R. Su, J. Xing, Q. Zhang, and Q. Xiong, “Metal halide perovskite nanomaterials: synthesis and applications,” Chem. Sci. (Camb.) 8(4), 2522–2536 (2017).
[Crossref] [PubMed]

K. Susumu, L. D. Field, E. Oh, M. Hunt, J. B. Delehanty, V. Palomo, P. E. Dawson, A. L. Huston, and I. L. Medintz, “Purple-, blue-, and green-emitting multishell alloyed quantum dots: synthesis, characterization, and application for ratiometric extracellular pH sensing,” Chem. Mater. 29(17), 7330–7344 (2017).
[Crossref]

2016 (9)

M. Auf der Maur, A. Pecchia, G. Penazzi, W. Rodrigues, and A. Di Carlo, “Efficiency drop in green InGaN/GaN light emitting diodes: the role of random alloy fluctuations,” Phys. Rev. Lett. 116(2), 027401 (2016).
[Crossref] [PubMed]

B. R. Sutherland and E. H. Sargent, “Perovskite photonic sources,” Nat. Photonics 10(5), 295–302 (2016).
[Crossref]

Q. Zhang, R. Su, X. Liu, J. Xing, T. C. Sum, and Q. Xiong, “High-quality whispering-gallery-mode lasing from cesium lead halide perovskite nanoplatelets,” Adv. Funct. Mater. 26(34), 6238–6245 (2016).
[Crossref]

Z. Wei, A. Perumal, R. Su, S. Sushant, J. Xing, Q. Zhang, S. T. Tan, H. V. Demir, and Q. Xiong, “Solution-processed highly bright and durable cesium lead halide perovskite light-emitting diodes,” Nanoscale 8(42), 18021–18026 (2016).
[Crossref] [PubMed]

Y. Fu, H. Zhu, C. C. Stoumpos, Q. Ding, J. Wang, M. G. Kanatzidis, X. Zhu, and S. Jin, “Broad wavelength tunable robust lasing from single-crystal nanowires of cesium lead halide perovskites (CsPbX 3, X = Cl, Br, I),” ACS Nano 10(8), 7963–7972 (2016).
[Crossref] [PubMed]

S. W. Eaton, M. Lai, N. A. Gibson, A. B. Wong, L. Dou, J. Ma, L.-W. Wang, S. R. Leone, and P. Yang, “Lasing in robust cesium lead halide perovskite nanowires,” Proc. Natl. Acad. Sci. U.S.A. 113(8), 1993–1998 (2016).
[Crossref] [PubMed]

S. Chen, K. Roh, J. Lee, W. K. Chong, Y. Lu, N. Mathews, T. C. Sum, and A. Nurmikko, “A photonic crystal laser from solution based organo-lead iodide perovskite thin films,” ACS Nano 10(4), 3959–3967 (2016).
[Crossref] [PubMed]

Y. Xu, Q. Chen, C. Zhang, R. Wang, H. Wu, X. Zhang, G. Xing, W. W. Yu, X. Wang, Y. Zhang, and M. Xiao, “Two-photon-pumped perovskite semiconductor nanocrystal lasers,” J. Am. Chem. Soc. 138(11), 3761–3768 (2016).
[Crossref] [PubMed]

N. S. Makarov, S. Guo, O. Isaienko, W. Liu, I. Robel, and V. I. Klimov, “Spectral and dynamical properties of single excitons, biexcitons, and trions in cesium–lead-halide perovskite quantum dots,” Nano Lett. 16(4), 2349–2362 (2016).
[Crossref] [PubMed]

2015 (7)

L. Protesescu, S. Yakunin, M. I. Bodnarchuk, F. Krieg, R. Caputo, C. H. Hendon, R. X. Yang, A. Walsh, and M. V. Kovalenko, “Nanocrystals of cesium lead halide perovskites (CsPbX3, X = Cl, Br, and I): novel optoelectronic materials showing bright emission with wide color gamut,” Nano Lett. 15(6), 3692–3696 (2015).
[Crossref] [PubMed]

K. Chen and H. Tüysüz, “Morphology-controlled synthesis of organometal halide perovskite inverse opals,” Angew. Chem. Int. Ed. Engl. 54(46), 13806–13810 (2015).
[Crossref] [PubMed]

H. Zhu, Y. Fu, F. Meng, X. Wu, Z. Gong, Q. Ding, M. V. Gustafsson, M. T. Trinh, S. Jin, and X.-Y. Zhu, “Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors,” Nat. Mater. 14(6), 636–642 (2015).
[Crossref] [PubMed]

Y. Wang, X. Li, J. Song, L. Xiao, H. Zeng, and H. Sun, “All-inorganic colloidal perovskite quantum dots: a new class of lasing materials with favorable characteristics,” Adv. Mater. 27(44), 7101–7108 (2015).
[Crossref] [PubMed]

S. Yakunin, L. Protesescu, F. Krieg, M. I. Bodnarchuk, G. Nedelcu, M. Humer, G. De Luca, M. Fiebig, W. Heiss, and M. V. Kovalenko, “Low-threshold amplified spontaneous emission and lasing from colloidal nanocrystals of caesium lead halide perovskites,” Nat. Commun. 6(1), 8056 (2015).
[Crossref] [PubMed]

J. Xing, X. F. Liu, Q. Zhang, S. T. Ha, Y. W. Yuan, C. Shen, T. C. Sum, and Q. Xiong, “Vapor phase synthesis of organometal halide perovskite nanowires for tunable room-temperature nanolasers,” Nano Lett. 15(7), 4571–4577 (2015).
[Crossref] [PubMed]

R. E. Brandt, V. Stevanović, D. S. Ginley, and T. Buonassisi, “Identifying defect-tolerant semiconductors with high minority-carrier lifetimes: beyond hybrid lead halide perovskites,” MRS Commun. 5(2), 265–275 (2015).
[Crossref]

2014 (4)

G. Xing, N. Mathews, S. S. Lim, N. Yantara, X. Liu, D. Sabba, M. Grätzel, S. Mhaisalkar, and T. C. Sum, “Low-temperature solution-processed wavelength-tunable perovskites for lasing,” Nat. Mater. 13(5), 476–480 (2014).
[Crossref] [PubMed]

J. Q. Grim, S. Christodoulou, F. Di Stasio, R. Krahne, R. Cingolani, L. Manna, and I. Moreels, “Continuous-wave biexciton lasing at room temperature using solution-processed quantum wells,” Nat. Nanotechnol. 9(11), 891–895 (2014).
[Crossref] [PubMed]

M. A. Green, A. Ho-Baillie, and H. J. Snaith, “The emergence of perovskite solar cells,” Nat. Photonics 8(7), 506–514 (2014).
[Crossref]

Q. Zhang, S. T. Ha, X. Liu, T. C. Sum, and Q. Xiong, “Room-Temperature Near-Infrared High-Q Perovskite Whispering-Gallery Planar Nanolasers,” Nano Lett. 14(10), 5995–6001 (2014).
[Crossref] [PubMed]

2012 (1)

E. Taylor, P. R. Edwards, and R. W. Martin, “Colorimetry and efficiency of white LEDs: Spectral width dependence,” Phys. Status Solidi., A Appl. Mater. Sci. 209(3), 461–464 (2012).
[Crossref]

2010 (1)

A. F. Oskooi, D. Roundy, M. Ibanescu, P. Bermel, J. D. Joannopoulos, and S. G. Johnson, “Meep: A flexible free-software package for electromagnetic simulations by the FDTD method,” Comput. Phys. Commun. 181(3), 687–702 (2010).
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2007 (1)

V. I. Klimov, “Spectral and dynamical properties of multiexcitons in semiconductor nanocrystals,” Annu. Rev. Phys. Chem. 58(1), 635–673 (2007).
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1996 (1)

M. P. van Exter, G. Nienhuis, and J. P. Woerdman, “Two simple expressions for the spontaneous emission factor B,” Phys. Rev. B Condens. Matter 54, 6 (1996).

Alsaedi, A.

S. Ma, M. Cai, T. Cheng, X. Ding, X. Shi, A. Alsaedi, T. Hayat, Y. Ding, Z. Tan, and S. Dai, “Two-dimensional organic-inorganic hybrid perovskite: from material properties to device applications,” Sci. China Mater. 61(10), 1257–1277 (2018).
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Auf der Maur, M.

M. Auf der Maur, A. Pecchia, G. Penazzi, W. Rodrigues, and A. Di Carlo, “Efficiency drop in green InGaN/GaN light emitting diodes: the role of random alloy fluctuations,” Phys. Rev. Lett. 116(2), 027401 (2016).
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Becker, M. A.

M. A. Becker, R. Vaxenburg, G. Nedelcu, P. C. Sercel, A. Shabaev, M. J. Mehl, J. G. Michopoulos, S. G. Lambrakos, N. Bernstein, J. L. Lyons, T. Stöferle, R. F. Mahrt, M. V. Kovalenko, D. J. Norris, G. Rainò, and A. L. Efros, “Bright triplet excitons in caesium lead halide perovskites,” Nature 553(7687), 189–193 (2018).
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Bermel, P.

A. F. Oskooi, D. Roundy, M. Ibanescu, P. Bermel, J. D. Joannopoulos, and S. G. Johnson, “Meep: A flexible free-software package for electromagnetic simulations by the FDTD method,” Comput. Phys. Commun. 181(3), 687–702 (2010).
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Bernstein, N.

M. A. Becker, R. Vaxenburg, G. Nedelcu, P. C. Sercel, A. Shabaev, M. J. Mehl, J. G. Michopoulos, S. G. Lambrakos, N. Bernstein, J. L. Lyons, T. Stöferle, R. F. Mahrt, M. V. Kovalenko, D. J. Norris, G. Rainò, and A. L. Efros, “Bright triplet excitons in caesium lead halide perovskites,” Nature 553(7687), 189–193 (2018).
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Bodnarchuk, M. I.

Z. Yang, M. Pelton, M. I. Bodnarchuk, M. V. Kovalenko, and E. Waks, “Spontaneous emission enhancement of colloidal perovskite nanocrystals by a photonic crystal cavity,” Appl. Phys. Lett. 111(22), 221104 (2017).
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L. Protesescu, S. Yakunin, M. I. Bodnarchuk, F. Krieg, R. Caputo, C. H. Hendon, R. X. Yang, A. Walsh, and M. V. Kovalenko, “Nanocrystals of cesium lead halide perovskites (CsPbX3, X = Cl, Br, and I): novel optoelectronic materials showing bright emission with wide color gamut,” Nano Lett. 15(6), 3692–3696 (2015).
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S. Yakunin, L. Protesescu, F. Krieg, M. I. Bodnarchuk, G. Nedelcu, M. Humer, G. De Luca, M. Fiebig, W. Heiss, and M. V. Kovalenko, “Low-threshold amplified spontaneous emission and lasing from colloidal nanocrystals of caesium lead halide perovskites,” Nat. Commun. 6(1), 8056 (2015).
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Brandt, R. E.

R. E. Brandt, V. Stevanović, D. S. Ginley, and T. Buonassisi, “Identifying defect-tolerant semiconductors with high minority-carrier lifetimes: beyond hybrid lead halide perovskites,” MRS Commun. 5(2), 265–275 (2015).
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Brittman, S.

S. Schünemann, S. Brittman, K. Chen, E. C. Garnett, and H. Tüysüz, “Halide perovskite 3D photonic crystals for distributed feedback lasers,” ACS Photonics 4(10), 2522–2528 (2017).
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Buonassisi, T.

R. E. Brandt, V. Stevanović, D. S. Ginley, and T. Buonassisi, “Identifying defect-tolerant semiconductors with high minority-carrier lifetimes: beyond hybrid lead halide perovskites,” MRS Commun. 5(2), 265–275 (2015).
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Cai, B.

B. Cai, X. Li, Y. Gu, M. Harb, J. Li, M. Xie, F. Cao, J. Song, S. Zhang, L. Cavallo, and H. Zeng, “Quantum confinement effect of two-dimensional all-inorganic halide perovskites,” Sci. China Mater. 60(9), 811–818 (2017).
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Cai, M.

S. Ma, M. Cai, T. Cheng, X. Ding, X. Shi, A. Alsaedi, T. Hayat, Y. Ding, Z. Tan, and S. Dai, “Two-dimensional organic-inorganic hybrid perovskite: from material properties to device applications,” Sci. China Mater. 61(10), 1257–1277 (2018).
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Cao, F.

B. Cai, X. Li, Y. Gu, M. Harb, J. Li, M. Xie, F. Cao, J. Song, S. Zhang, L. Cavallo, and H. Zeng, “Quantum confinement effect of two-dimensional all-inorganic halide perovskites,” Sci. China Mater. 60(9), 811–818 (2017).
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Caputo, R.

L. Protesescu, S. Yakunin, M. I. Bodnarchuk, F. Krieg, R. Caputo, C. H. Hendon, R. X. Yang, A. Walsh, and M. V. Kovalenko, “Nanocrystals of cesium lead halide perovskites (CsPbX3, X = Cl, Br, and I): novel optoelectronic materials showing bright emission with wide color gamut,” Nano Lett. 15(6), 3692–3696 (2015).
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Cavallo, L.

B. Cai, X. Li, Y. Gu, M. Harb, J. Li, M. Xie, F. Cao, J. Song, S. Zhang, L. Cavallo, and H. Zeng, “Quantum confinement effect of two-dimensional all-inorganic halide perovskites,” Sci. China Mater. 60(9), 811–818 (2017).
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Chen, J.

Y. Fu, H. Zhu, J. Chen, M. P. Hautzinger, X.-Y. Zhu, and S. Jin, “Metal halide perovskite nanostructures for optoelectronic applications and the study of physical properties,” Nat. Rev. Mater. 4(3), 169–188 (2019).
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J. Wu, J. Chen, Y. Zhang, Z. Xu, L. Zhao, T. Liu, D. Luo, W. Yang, K. Chen, Q. Hu, F. Ye, P. Wu, R. Zhu, and Q. Gong, “Pinhole-free hybrid perovskite film with arbitrarily-shaped micro-patterns for functional optoelectronic devices,” Nano Lett. 17(6), 3563–3569 (2017).
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Chen, K.

J. Wu, J. Chen, Y. Zhang, Z. Xu, L. Zhao, T. Liu, D. Luo, W. Yang, K. Chen, Q. Hu, F. Ye, P. Wu, R. Zhu, and Q. Gong, “Pinhole-free hybrid perovskite film with arbitrarily-shaped micro-patterns for functional optoelectronic devices,” Nano Lett. 17(6), 3563–3569 (2017).
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S. Schünemann, S. Brittman, K. Chen, E. C. Garnett, and H. Tüysüz, “Halide perovskite 3D photonic crystals for distributed feedback lasers,” ACS Photonics 4(10), 2522–2528 (2017).
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K. Chen and H. Tüysüz, “Morphology-controlled synthesis of organometal halide perovskite inverse opals,” Angew. Chem. Int. Ed. Engl. 54(46), 13806–13810 (2015).
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Chen, L.

C. Yin, L. Chen, N. Song, Y. Lv, F. Hu, C. Sun, W. W. Yu, C. Zhang, X. Wang, Y. Zhang, and M. Xiao, “Bright-exciton fine-structure splittings in single perovskite nanocrystals,” Phys. Rev. Lett. 119(2), 026401 (2017).
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Chen, Q.

Y. Xu, Q. Chen, C. Zhang, R. Wang, H. Wu, X. Zhang, G. Xing, W. W. Yu, X. Wang, Y. Zhang, and M. Xiao, “Two-photon-pumped perovskite semiconductor nanocrystal lasers,” J. Am. Chem. Soc. 138(11), 3761–3768 (2016).
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Chen, S.

F. Yan, J. Xing, G. Xing, L. Quan, S. T. Tan, J. Zhao, R. Su, L. Zhang, S. Chen, Y. Zhao, A. Huan, E. H. Sargent, Q. Xiong, and H. V. Demir, “Highly Efficient Visible Colloidal Lead-Halide Perovskite Nanocrystal Light-Emitting Diodes,” Nano Lett. 18(5), 3157–3164 (2018).
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S. Chen, K. Roh, J. Lee, W. K. Chong, Y. Lu, N. Mathews, T. C. Sum, and A. Nurmikko, “A photonic crystal laser from solution based organo-lead iodide perovskite thin films,” ACS Nano 10(4), 3959–3967 (2016).
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Chen, Y.

Y. Chen, A. Ryou, M. R. Friedfeld, T. Fryett, J. Whitehead, B. M. Cossairt, and A. Majumdar, “Deterministic positioning of colloidal quantum dots on silicon nitride nanobeam cavities,” Nano Lett. 18(10), 6404–6410 (2018).
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T. K. Fryett, Y. Chen, J. Whitehead, Z. M. Peycke, X. Xu, and A. Majumdar, “Encapsulated silicon nitride nanobeam cavity for hybrid nanophotonics,” ACS Photonics 5(6), 2176–2181 (2018).
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Chen, Z.

R. Su, C. Diederichs, J. Wang, T. C. H. Liew, J. Zhao, S. Liu, W. Xu, Z. Chen, and Q. Xiong, “Room-temperature polariton lasing in all-inorganic perovskite nanoplatelets,” Nano Lett. 17(6), 3982–3988 (2017).
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Cheng, T.

S. Ma, M. Cai, T. Cheng, X. Ding, X. Shi, A. Alsaedi, T. Hayat, Y. Ding, Z. Tan, and S. Dai, “Two-dimensional organic-inorganic hybrid perovskite: from material properties to device applications,” Sci. China Mater. 61(10), 1257–1277 (2018).
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Chong, W. K.

S. Chen, K. Roh, J. Lee, W. K. Chong, Y. Lu, N. Mathews, T. C. Sum, and A. Nurmikko, “A photonic crystal laser from solution based organo-lead iodide perovskite thin films,” ACS Nano 10(4), 3959–3967 (2016).
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Christodoulou, S.

J. Q. Grim, S. Christodoulou, F. Di Stasio, R. Krahne, R. Cingolani, L. Manna, and I. Moreels, “Continuous-wave biexciton lasing at room temperature using solution-processed quantum wells,” Nat. Nanotechnol. 9(11), 891–895 (2014).
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Cingolani, R.

J. Q. Grim, S. Christodoulou, F. Di Stasio, R. Krahne, R. Cingolani, L. Manna, and I. Moreels, “Continuous-wave biexciton lasing at room temperature using solution-processed quantum wells,” Nat. Nanotechnol. 9(11), 891–895 (2014).
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Cossairt, B. M.

Y. Chen, A. Ryou, M. R. Friedfeld, T. Fryett, J. Whitehead, B. M. Cossairt, and A. Majumdar, “Deterministic positioning of colloidal quantum dots on silicon nitride nanobeam cavities,” Nano Lett. 18(10), 6404–6410 (2018).
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Cui, C.

T. Thu Ha Do, A. Granados del Águila, C. Cui, J. Xing, Z. Ning, and Q. Xiong, “Optical study on intrinsic exciton states in high-quality CH3NH3PbBr3 single crystals,” Phys. Rev. B 96(7), 075308 (2017).
[Crossref]

Dai, S.

S. Ma, M. Cai, T. Cheng, X. Ding, X. Shi, A. Alsaedi, T. Hayat, Y. Ding, Z. Tan, and S. Dai, “Two-dimensional organic-inorganic hybrid perovskite: from material properties to device applications,” Sci. China Mater. 61(10), 1257–1277 (2018).
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Dawson, P. E.

K. Susumu, L. D. Field, E. Oh, M. Hunt, J. B. Delehanty, V. Palomo, P. E. Dawson, A. L. Huston, and I. L. Medintz, “Purple-, blue-, and green-emitting multishell alloyed quantum dots: synthesis, characterization, and application for ratiometric extracellular pH sensing,” Chem. Mater. 29(17), 7330–7344 (2017).
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de Arquer, F. P. G.

K. Lin, J. Xing, L. N. Quan, F. P. G. de Arquer, X. Gong, J. Lu, L. Xie, W. Zhao, D. Zhang, C. Yan, W. Li, X. Liu, Y. Lu, J. Kirman, E. H. Sargent, Q. Xiong, and Z. Wei, “Perovskite light-emitting diodes with external quantum efficiency exceeding 20 per cent,” Nature 562(7726), 245–248 (2018).
[Crossref] [PubMed]

De Luca, G.

S. Yakunin, L. Protesescu, F. Krieg, M. I. Bodnarchuk, G. Nedelcu, M. Humer, G. De Luca, M. Fiebig, W. Heiss, and M. V. Kovalenko, “Low-threshold amplified spontaneous emission and lasing from colloidal nanocrystals of caesium lead halide perovskites,” Nat. Commun. 6(1), 8056 (2015).
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Delehanty, J. B.

K. Susumu, L. D. Field, E. Oh, M. Hunt, J. B. Delehanty, V. Palomo, P. E. Dawson, A. L. Huston, and I. L. Medintz, “Purple-, blue-, and green-emitting multishell alloyed quantum dots: synthesis, characterization, and application for ratiometric extracellular pH sensing,” Chem. Mater. 29(17), 7330–7344 (2017).
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Demir, H. V.

F. Yan, J. Xing, G. Xing, L. Quan, S. T. Tan, J. Zhao, R. Su, L. Zhang, S. Chen, Y. Zhao, A. Huan, E. H. Sargent, Q. Xiong, and H. V. Demir, “Highly Efficient Visible Colloidal Lead-Halide Perovskite Nanocrystal Light-Emitting Diodes,” Nano Lett. 18(5), 3157–3164 (2018).
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Z. Wei, A. Perumal, R. Su, S. Sushant, J. Xing, Q. Zhang, S. T. Tan, H. V. Demir, and Q. Xiong, “Solution-processed highly bright and durable cesium lead halide perovskite light-emitting diodes,” Nanoscale 8(42), 18021–18026 (2016).
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Di Carlo, A.

M. Auf der Maur, A. Pecchia, G. Penazzi, W. Rodrigues, and A. Di Carlo, “Efficiency drop in green InGaN/GaN light emitting diodes: the role of random alloy fluctuations,” Phys. Rev. Lett. 116(2), 027401 (2016).
[Crossref] [PubMed]

Di Stasio, F.

J. Q. Grim, S. Christodoulou, F. Di Stasio, R. Krahne, R. Cingolani, L. Manna, and I. Moreels, “Continuous-wave biexciton lasing at room temperature using solution-processed quantum wells,” Nat. Nanotechnol. 9(11), 891–895 (2014).
[Crossref] [PubMed]

Diederichs, C.

R. Su, C. Diederichs, J. Wang, T. C. H. Liew, J. Zhao, S. Liu, W. Xu, Z. Chen, and Q. Xiong, “Room-temperature polariton lasing in all-inorganic perovskite nanoplatelets,” Nano Lett. 17(6), 3982–3988 (2017).
[Crossref] [PubMed]

Ding, Q.

Y. Fu, H. Zhu, C. C. Stoumpos, Q. Ding, J. Wang, M. G. Kanatzidis, X. Zhu, and S. Jin, “Broad wavelength tunable robust lasing from single-crystal nanowires of cesium lead halide perovskites (CsPbX 3, X = Cl, Br, I),” ACS Nano 10(8), 7963–7972 (2016).
[Crossref] [PubMed]

H. Zhu, Y. Fu, F. Meng, X. Wu, Z. Gong, Q. Ding, M. V. Gustafsson, M. T. Trinh, S. Jin, and X.-Y. Zhu, “Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors,” Nat. Mater. 14(6), 636–642 (2015).
[Crossref] [PubMed]

Ding, X.

S. Ma, M. Cai, T. Cheng, X. Ding, X. Shi, A. Alsaedi, T. Hayat, Y. Ding, Z. Tan, and S. Dai, “Two-dimensional organic-inorganic hybrid perovskite: from material properties to device applications,” Sci. China Mater. 61(10), 1257–1277 (2018).
[Crossref]

Ding, Y.

S. Ma, M. Cai, T. Cheng, X. Ding, X. Shi, A. Alsaedi, T. Hayat, Y. Ding, Z. Tan, and S. Dai, “Two-dimensional organic-inorganic hybrid perovskite: from material properties to device applications,” Sci. China Mater. 61(10), 1257–1277 (2018).
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Dou, L.

S. W. Eaton, M. Lai, N. A. Gibson, A. B. Wong, L. Dou, J. Ma, L.-W. Wang, S. R. Leone, and P. Yang, “Lasing in robust cesium lead halide perovskite nanowires,” Proc. Natl. Acad. Sci. U.S.A. 113(8), 1993–1998 (2016).
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Du, W.

Q. Zhang, R. Su, W. Du, X. Liu, L. Zhao, S. T. Ha, and Q. Xiong, “Advances in Small Perovskite-Based Lasers,” Small Methods 1(9), 1700163 (2017).
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Eaton, S. W.

S. W. Eaton, M. Lai, N. A. Gibson, A. B. Wong, L. Dou, J. Ma, L.-W. Wang, S. R. Leone, and P. Yang, “Lasing in robust cesium lead halide perovskite nanowires,” Proc. Natl. Acad. Sci. U.S.A. 113(8), 1993–1998 (2016).
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Edwards, P. R.

E. Taylor, P. R. Edwards, and R. W. Martin, “Colorimetry and efficiency of white LEDs: Spectral width dependence,” Phys. Status Solidi., A Appl. Mater. Sci. 209(3), 461–464 (2012).
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Efros, A. L.

M. A. Becker, R. Vaxenburg, G. Nedelcu, P. C. Sercel, A. Shabaev, M. J. Mehl, J. G. Michopoulos, S. G. Lambrakos, N. Bernstein, J. L. Lyons, T. Stöferle, R. F. Mahrt, M. V. Kovalenko, D. J. Norris, G. Rainò, and A. L. Efros, “Bright triplet excitons in caesium lead halide perovskites,” Nature 553(7687), 189–193 (2018).
[Crossref] [PubMed]

Fiebig, M.

S. Yakunin, L. Protesescu, F. Krieg, M. I. Bodnarchuk, G. Nedelcu, M. Humer, G. De Luca, M. Fiebig, W. Heiss, and M. V. Kovalenko, “Low-threshold amplified spontaneous emission and lasing from colloidal nanocrystals of caesium lead halide perovskites,” Nat. Commun. 6(1), 8056 (2015).
[Crossref] [PubMed]

Field, L. D.

K. Susumu, L. D. Field, E. Oh, M. Hunt, J. B. Delehanty, V. Palomo, P. E. Dawson, A. L. Huston, and I. L. Medintz, “Purple-, blue-, and green-emitting multishell alloyed quantum dots: synthesis, characterization, and application for ratiometric extracellular pH sensing,” Chem. Mater. 29(17), 7330–7344 (2017).
[Crossref]

Friedfeld, M. R.

Y. Chen, A. Ryou, M. R. Friedfeld, T. Fryett, J. Whitehead, B. M. Cossairt, and A. Majumdar, “Deterministic positioning of colloidal quantum dots on silicon nitride nanobeam cavities,” Nano Lett. 18(10), 6404–6410 (2018).
[Crossref] [PubMed]

Fryett, T.

Y. Chen, A. Ryou, M. R. Friedfeld, T. Fryett, J. Whitehead, B. M. Cossairt, and A. Majumdar, “Deterministic positioning of colloidal quantum dots on silicon nitride nanobeam cavities,” Nano Lett. 18(10), 6404–6410 (2018).
[Crossref] [PubMed]

Fryett, T. K.

T. K. Fryett, Y. Chen, J. Whitehead, Z. M. Peycke, X. Xu, and A. Majumdar, “Encapsulated silicon nitride nanobeam cavity for hybrid nanophotonics,” ACS Photonics 5(6), 2176–2181 (2018).
[Crossref]

Fu, Y.

Y. Fu, H. Zhu, J. Chen, M. P. Hautzinger, X.-Y. Zhu, and S. Jin, “Metal halide perovskite nanostructures for optoelectronic applications and the study of physical properties,” Nat. Rev. Mater. 4(3), 169–188 (2019).
[Crossref]

Y. Fu, H. Zhu, C. C. Stoumpos, Q. Ding, J. Wang, M. G. Kanatzidis, X. Zhu, and S. Jin, “Broad wavelength tunable robust lasing from single-crystal nanowires of cesium lead halide perovskites (CsPbX 3, X = Cl, Br, I),” ACS Nano 10(8), 7963–7972 (2016).
[Crossref] [PubMed]

H. Zhu, Y. Fu, F. Meng, X. Wu, Z. Gong, Q. Ding, M. V. Gustafsson, M. T. Trinh, S. Jin, and X.-Y. Zhu, “Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors,” Nat. Mater. 14(6), 636–642 (2015).
[Crossref] [PubMed]

Garnett, E. C.

S. Schünemann, S. Brittman, K. Chen, E. C. Garnett, and H. Tüysüz, “Halide perovskite 3D photonic crystals for distributed feedback lasers,” ACS Photonics 4(10), 2522–2528 (2017).
[Crossref]

Gibson, N. A.

S. W. Eaton, M. Lai, N. A. Gibson, A. B. Wong, L. Dou, J. Ma, L.-W. Wang, S. R. Leone, and P. Yang, “Lasing in robust cesium lead halide perovskite nanowires,” Proc. Natl. Acad. Sci. U.S.A. 113(8), 1993–1998 (2016).
[Crossref] [PubMed]

Ginley, D. S.

R. E. Brandt, V. Stevanović, D. S. Ginley, and T. Buonassisi, “Identifying defect-tolerant semiconductors with high minority-carrier lifetimes: beyond hybrid lead halide perovskites,” MRS Commun. 5(2), 265–275 (2015).
[Crossref]

Gong, Q.

J. Wu, J. Chen, Y. Zhang, Z. Xu, L. Zhao, T. Liu, D. Luo, W. Yang, K. Chen, Q. Hu, F. Ye, P. Wu, R. Zhu, and Q. Gong, “Pinhole-free hybrid perovskite film with arbitrarily-shaped micro-patterns for functional optoelectronic devices,” Nano Lett. 17(6), 3563–3569 (2017).
[Crossref] [PubMed]

Gong, X.

K. Lin, J. Xing, L. N. Quan, F. P. G. de Arquer, X. Gong, J. Lu, L. Xie, W. Zhao, D. Zhang, C. Yan, W. Li, X. Liu, Y. Lu, J. Kirman, E. H. Sargent, Q. Xiong, and Z. Wei, “Perovskite light-emitting diodes with external quantum efficiency exceeding 20 per cent,” Nature 562(7726), 245–248 (2018).
[Crossref] [PubMed]

Gong, Z.

H. Zhu, Y. Fu, F. Meng, X. Wu, Z. Gong, Q. Ding, M. V. Gustafsson, M. T. Trinh, S. Jin, and X.-Y. Zhu, “Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors,” Nat. Mater. 14(6), 636–642 (2015).
[Crossref] [PubMed]

Granados del Águila, A.

T. Thu Ha Do, A. Granados del Águila, C. Cui, J. Xing, Z. Ning, and Q. Xiong, “Optical study on intrinsic exciton states in high-quality CH3NH3PbBr3 single crystals,” Phys. Rev. B 96(7), 075308 (2017).
[Crossref]

Grätzel, M.

G. Xing, N. Mathews, S. S. Lim, N. Yantara, X. Liu, D. Sabba, M. Grätzel, S. Mhaisalkar, and T. C. Sum, “Low-temperature solution-processed wavelength-tunable perovskites for lasing,” Nat. Mater. 13(5), 476–480 (2014).
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Green, M. A.

M. A. Green, A. Ho-Baillie, and H. J. Snaith, “The emergence of perovskite solar cells,” Nat. Photonics 8(7), 506–514 (2014).
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Grim, J. Q.

J. Q. Grim, S. Christodoulou, F. Di Stasio, R. Krahne, R. Cingolani, L. Manna, and I. Moreels, “Continuous-wave biexciton lasing at room temperature using solution-processed quantum wells,” Nat. Nanotechnol. 9(11), 891–895 (2014).
[Crossref] [PubMed]

Gu, Y.

B. Cai, X. Li, Y. Gu, M. Harb, J. Li, M. Xie, F. Cao, J. Song, S. Zhang, L. Cavallo, and H. Zeng, “Quantum confinement effect of two-dimensional all-inorganic halide perovskites,” Sci. China Mater. 60(9), 811–818 (2017).
[Crossref]

Guo, S.

N. S. Makarov, S. Guo, O. Isaienko, W. Liu, I. Robel, and V. I. Klimov, “Spectral and dynamical properties of single excitons, biexcitons, and trions in cesium–lead-halide perovskite quantum dots,” Nano Lett. 16(4), 2349–2362 (2016).
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Gustafsson, M. V.

H. Zhu, Y. Fu, F. Meng, X. Wu, Z. Gong, Q. Ding, M. V. Gustafsson, M. T. Trinh, S. Jin, and X.-Y. Zhu, “Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors,” Nat. Mater. 14(6), 636–642 (2015).
[Crossref] [PubMed]

Ha, S. T.

Q. Zhang, R. Su, W. Du, X. Liu, L. Zhao, S. T. Ha, and Q. Xiong, “Advances in Small Perovskite-Based Lasers,” Small Methods 1(9), 1700163 (2017).
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J. Xing, X. F. Liu, Q. Zhang, S. T. Ha, Y. W. Yuan, C. Shen, T. C. Sum, and Q. Xiong, “Vapor phase synthesis of organometal halide perovskite nanowires for tunable room-temperature nanolasers,” Nano Lett. 15(7), 4571–4577 (2015).
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K. Susumu, L. D. Field, E. Oh, M. Hunt, J. B. Delehanty, V. Palomo, P. E. Dawson, A. L. Huston, and I. L. Medintz, “Purple-, blue-, and green-emitting multishell alloyed quantum dots: synthesis, characterization, and application for ratiometric extracellular pH sensing,” Chem. Mater. 29(17), 7330–7344 (2017).
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H. Zhu, Y. Fu, F. Meng, X. Wu, Z. Gong, Q. Ding, M. V. Gustafsson, M. T. Trinh, S. Jin, and X.-Y. Zhu, “Lead halide perovskite nanowire lasers with low lasing thresholds and high quality factors,” Nat. Mater. 14(6), 636–642 (2015).
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F. Yan, J. Xing, G. Xing, L. Quan, S. T. Tan, J. Zhao, R. Su, L. Zhang, S. Chen, Y. Zhao, A. Huan, E. H. Sargent, Q. Xiong, and H. V. Demir, “Highly Efficient Visible Colloidal Lead-Halide Perovskite Nanocrystal Light-Emitting Diodes,” Nano Lett. 18(5), 3157–3164 (2018).
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ACS Nano (2)

Y. Fu, H. Zhu, C. C. Stoumpos, Q. Ding, J. Wang, M. G. Kanatzidis, X. Zhu, and S. Jin, “Broad wavelength tunable robust lasing from single-crystal nanowires of cesium lead halide perovskites (CsPbX 3, X = Cl, Br, I),” ACS Nano 10(8), 7963–7972 (2016).
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Nanoscale (1)

Z. Wei, A. Perumal, R. Su, S. Sushant, J. Xing, Q. Zhang, S. T. Tan, H. V. Demir, and Q. Xiong, “Solution-processed highly bright and durable cesium lead halide perovskite light-emitting diodes,” Nanoscale 8(42), 18021–18026 (2016).
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Figures (5)

Fig. 1
Fig. 1 Schematic of the perovskite nanocrystal coupled SiN nanobeam photonic crystal cavity. (a) 3D rendering of the SiN nanobeam on a substrate encapsulated with a PMMA layer mixed with perovskite nanocrystal as labelled. The SiN nanobeam sits on top of an oxide substrate giving it mechanical robustness. (b) A cross-sectional view along the length of the nanobeam illustrating the various materials with the colors indicating the respective material index. Here, the PMMA layer is set to have an index of 1.6 to distinguish it from the substrate with index of 1.45. The thickness of the PMMA layer in the FDTD simulation is the length from the surface of the substrate to the top of the PMMA layer. The holes of the nanobeam are taken to be filled with material of the same index as that of the PMMA layer.
Fig. 2
Fig. 2 Characteristics of the SiN nanobeam. (a) Schematic of the nanobeam with elliptical holes with the parameters period, a and width labelled. The cavity is formed by linearly reducing both the hole period and the major axis of the 10 holes at the center on each side of the nanobeam as indicated by the dashed arrows (see main text for the parameter values). (b) Simulated electric field intensity distribution of the fundamental cavity mode. (c) Scanning electron micrograph (SEM) of the PMMA encapsulated SiN nanobeam. As the PMMA layer is nonconductive, the resulting SEM image is less sharp. Nonetheless, the edges of the nanobeam, as well as the linearly decreasing hole sizes can be clearly seen in the image.
Fig. 3
Fig. 3 Tuning of cavity mode resonance (a) A series of spectra under around 15 µW of CW laser excitation corresponding to the decreasing perovskite concentration in the direction of the dashed arrow. The spectra show the broad perovskite PL emission peak center at 520 nm and the narrow cavity mode resonances as indicated by the arrows along with the respective Q-factors. The mode resonant wavelength decreases with the decreasing concentration of perovskites in the PMMA layer. (b) The simulated cavity mode resonant wavelength (black squares) decreases with the decrease of the effective index of the PMMA layer, while the Q-factor (blue spheres) shows the opposite trend.
Fig. 4
Fig. 4 (a) The plot shows the change in the cavity mode wavelength with the effective index of the PMMA layer for different PMMA layer thicknesses, namely 250 nm, 400nm and 600nm. Depending on the actual thickness of the PMMA layers prepared experimentally, the cavity mode wavelength could take a value within the region marked in yellow. (b) As for the Q-factor, the thicker PMMA layers cause a drop in the Q-factors, with a larger effect at higher effective index.
Fig. 5
Fig. 5 Plot comparing the PL decay of the perovskite nanocrystals in two different cases: one which is coupled to the cavity (blue) and the other uncoupled (black) with the respective t 1 decay time as labelled.

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