Abstract

We report the measurement of the absolute frequencies of the 6s21S06s6p 3P1 transition (253.7 nm) and the relevant isotope shifts in five mercury isotopes  198Hg,  199Hg,  200Hg,  202Hg, and  204Hg. The Doppler-free saturated absorption measurements were performed in an atomic vapour cell at room temperature with a four-harmonic generated (FHG) continuous-wave (cw) laser digitally locked to the atomic transition. It was referenced with a femtosecond optical frequency comb synchronized to the frequency of local representation of the International Atomic Time to provide traceability to the SI second by the 330 km-long stabilized fibre optical link. The transition frequencies and isotope shifts have been determined with an accuracy of a few hundred kHz, at least one order of magnitude better than any previous measurement. By making a King plot with the isotope shifts of 6s6p 3P26s7s 3S1 transition (546 nm) we determined the accurate value of the ratio of the electronic field-shift parameters E546/E254 and estimated the electronic field-shift term E254.

© 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

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2018 (4)

M. S. Safronova, D. Budker, D. DeMille, D. F. J. Kimball, A. Derevianko, and C. W. Clark, “Search for new physics with atoms and molecules,” Rev. Mod. Phys. 90, 025008 (2018).
[Crossref]

V. V. Flambaum, A. J. Geddes, and A. V. Viatkina, “Isotope shift, nonlinearity of King plots, and the search for new particles,” Phys. Rev. A 97, 032510 (2018).
[Crossref]

J. C. Berengut, D. Budker, C. Delaunay, V. V. Flambaum, C. Frugiuele, E. Fuchs, C. Grojean, R. Harnik, R. Ozeri, G. Perez, and Y. Soreq, “Probing new long-range interactions by isotope shift spectroscopy,” Phys. Rev. Lett. 120, 091801 (2018).
[Crossref] [PubMed]

M. Witkowski, R. Munoz-Rodriguez, A. Raczyński, J. Zaremba, B. Nagórny, P. S. Żuchowski, R. Ciuryło, and M. Zawada, “Photoionization cross section of the  5S 1/2 and  5P 3/2 states of Rb in simultaneous magneto-optical trapping of Rb and Hg,” Phys. Rev. A 98, 053444 (2018).
[Crossref]

2017 (2)

2016 (1)

B. Graner, Y. Chen, E. G. Lindahl, and B. R. Heckel, “Reduced limit on the permanent electric dipole moment of  199Hg,” Phys. Rev. Lett. 116, 161601 (2016).
[Crossref]

2015 (3)

Z. Jiang, A. Czubla, J. Nawrocki, W. Lewandowski, and E. F. Arias, “Comparing a GPS time link calibration with an optical fibre self-calibration with 200 ps accuracy,” Metrologia 52(2), 384–391 (2015).
[Crossref]

P. Morzyński, M. Bober, D. Bartoszek-Bober, J. Nawrocki, P. Krehlik, L. Śliwczyński, M. Lipiński, P. Masłowski, A. Cygan, P. Dunst, M. Garus, D. Lisak, J. Zachorowski, W. Gawlik, C. Radzewicz, R. Ciuryło, and M. Zawada, “Absolute measurement of the  1S 0 -  3P 0 clock transition in neutral  88Sr over the 330 km-long stabilized fibre optic link,” Sci. Rep. 5, 17495 (2015).
[Crossref]

P. Krehlik, L. Śliwczyński, L. Buczek, J. Kołodziej, and M. Lipiński, “Ultrastable long-distance fibre-optic time transfer: active compensation over a wide range of delays,” Metrologia 52(1), 82–88 (2015).
[Crossref]

2013 (6)

L. Śliwczyński, P. Krehlik, A. Czubla, L. Buczek, and M. Lipiński, “Dissemination of time and RF frequency via a stabilized fibre optic link over a distance of 420 km,” Metrologia 50(2), 133–145 (2013).
[Crossref]

L. Hong-Li, Y. Shi-Qi, L. Kang-Kang, Q. Jun, X. Zhen, H. Tao, and W. Yu-Zhu, “Magneto-optical trap for neutral mercury atoms,” Chin. Phys. B 22(4), 043701 (2013).
[Crossref]

J. D. Deschênes and J. Genest, “Heterodyne beats between a continuous-wave laser and a frequency comb beyond the shot-noise limit of a single comb mode,” Phys. Rev. A 87, 023802 (2013).
[Crossref]

M. D. Swallows, T. H. Loftus, W. C. Griffith, B. R. Heckel, E. N. Fortson, and M. V. Romalis, “Techniques used to search for a permanent electric dipole moment of the  199Hg atom and the implications for CP violation,” Phys. Rev. A 87, 012102 (2013).
[Crossref]

P. Morzyński, P. Wcisło, P. Ablewski, R. Gartman, W. Gawlik, P. Masłowski, B. Nagórny, F. Ozimek, C. Radzewicz, M. Witkowski, R. Ciuryło, and M. Zawada, “Absolute frequency measurement of rubidium 5S - 7S two-photon transitions,” Opt. Lett. 38(22), 4581–4584 (2013).
[Crossref]

A. Cygan, D. Lisak, P. Morzyński, M. Bober, M. Zawada, E. Pazderski, and R. Ciuryło, “Cavity mode-width spectroscopy with widely tunable ultra narrow laser,” Opt. Express 21(24), 29744–29754 (2013).
[Crossref]

2011 (4)

S. Knecht, S. Fux, R. Van Meer, L. Visscher, M. Reiher, and T. Saue, “Mössbauer spectroscopy for heavy elements: a relativistic benchmark study of mercury,” Theor. Chem. Accounts 129(3–5), 631–650 (2011).
[Crossref]

A. E. Kramida, “Re-optimized energy levels and Ritz wavelengths of (198)Hg I,” J. Res. Natl. Inst. Stand. Technol. 116(2), 599–619 (2011).
[Crossref] [PubMed]

L. Yi, S. Mejri, J. J. McFerran, Y. Le Coq, and S. Bize, “Optical lattice trapping of  199Hg and determination of the magic wavelength for the ultraviolet  1S0↔3P0 clock transition,” Phys. Rev. Lett. 106, 073005 (2011).
[Crossref]

P. Villwock, S. Siol, and T. Walther, “Magneto-optical trapping of neutral mercury,” The Eur. Phys. J. D 65(1), 251–255 (2011).
[Crossref]

2010 (1)

C. J. Sansonetti and D. Veza, “Doppler-free measurement of the 546 nm line of mercury,” J. Phys. B: At. Mol. Opt. Phys. 43, 205003 (2010).
[Crossref]

2009 (2)

N. Shiga, Y. Li, H. Ito, S. Nagano, T. Ido, K. Bielska, R. S. Trawiński, and R. Ciuryło, “Buffer-gas-induced collision shift for the  88Sr 1S 0−3P 1 clock transition,” Phys. Rev. A 80, 030501 (2009).
[Crossref]

K. V. P. Latha, D. Angom, B. P. Das, and D. Mukherjee, “Probing CP violation with the electric dipole moment of atomic mercury,” Phys. Rev. Lett. 103, 083001 (2009).
[Crossref] [PubMed]

2008 (1)

H. Hachisu, K. Miyagishi, S. G. Porsev, A. Derevianko, V. D. Ovsiannikov, V. G. Pal’chikov, M. Takamoto, and H. Katori, “Trapping of neutral mercury atoms and prospects for optical lattice clocks,” Phys. Rev. Lett. 100,053001 (2008).
[Crossref] [PubMed]

2006 (3)

E. B. Saloman, “Wavelengths, energy level classifications, and energy levels for the spectrum of neutral mercury,” J. Phys. Chem. Ref. Data 35(4), 1519–1548 (2006).
[Crossref]

M. L. Huber, A. Laesecke, and D. G. Friend, “Correlation for the vapor pressure of mercury,” Ind. Eng. Chem. Res. 45(21), 7351–7361 (2006).
[Crossref]

R. Trawiński, “On argon-induced pressure shifts of  198Hg spectral lines associated with quasi-Rydberg transitions,” Acta Phys. Pol. A 110(1), 51–56 (2006).
[Crossref]

2005 (3)

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A. A. Hahn, J. P. Miller, R. J. Powers, A. Zehnder, A. M. Rushton, R. E. Welsh, A. R. Kunselman, P. Roberson, and H. K. Walter, “An experimental study of muonic x-ray transitions in mercury isotopes,” Nucl. Phys. A 314(2–3), 361–386 (1979).
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P. L. Lee, F. Boehm, and A. A. Hahn, “Variations of nuclear charge radii in mercury isotopes with A=198, 199, 200, 201, 202, and 204 from x-ray isotope shifts,” Phys. Rev. C 17(5), 1859–1861 (1978).
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S. Gerstenkorn, J. J. Labarthe, and J. Vergès, “Fine and hyperfine structures and isotope shifts in the arc spectrum of mercury. Part I. Experimental study of the infrared spectrum by Fourier transform spectroscopy,” Phys. Scripta 15(3), 167–172 (1977).
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C. V. Stager and R. H. Kohler, “Hyperfine structure of Hg 199 and Hg 201 in the  3P 1 state,” Bull. Am. Phys. Soc. Ser. II 5(4), 274 (1960).

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Adams, K. B.

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G. Ulm, S. K. Bhattacherjee, P. Dabkiewicz, G. Huber, H. J. Kluge, T. Kühl, H. Lochmann, E. W. Otten, K. Wendt, S. A. Ahmad, W. Klempt, R. Neugart, and ISOLDE Collaboration, “Isotope shift of  182Hg and an update of nuclear moments and charge radii in the isotope range  181Hg- 206Hg,” Zeitschrift für Physik A Atomic Nuclei 325(3), 247–259 (1986).
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N. Allard and J. Kielkopf, “The effect of neutral nonresonant collisions on atomic spectral lines,” Rev. Mod. Phys. 54(4), 1103–1182 (1982).
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Arias, E. F.

Z. Jiang, A. Czubla, J. Nawrocki, W. Lewandowski, and E. F. Arias, “Comparing a GPS time link calibration with an optical fibre self-calibration with 200 ps accuracy,” Metrologia 52(2), 384–391 (2015).
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E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

Autschbach, J.

E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

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J. Azoubib, J. Nawrocki, and W. Lewandowski, “Independent atomic timescale in Poland-organization and results,” Metrologia 40(3), S245–S248 (2003).
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E. van Lenthe, J. G. Snijders, and E. J. Baerends, “The zero-order regular approximation for relativistic effects: the effect of spin-orbit coupling in closed shell molecules,” J. Chem. Phys. 105(15), 6505–6516 (1996).
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Barger, R. L.

Bartoszek-Bober, D.

P. Morzyński, M. Bober, D. Bartoszek-Bober, J. Nawrocki, P. Krehlik, L. Śliwczyński, M. Lipiński, P. Masłowski, A. Cygan, P. Dunst, M. Garus, D. Lisak, J. Zachorowski, W. Gawlik, C. Radzewicz, R. Ciuryło, and M. Zawada, “Absolute measurement of the  1S 0 -  3P 0 clock transition in neutral  88Sr over the 330 km-long stabilized fibre optic link,” Sci. Rep. 5, 17495 (2015).
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E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

Bashford, D.

E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

Baylis, W.

J. Szudy and W. Baylis, “Asymmetry in pressure-broadened spectral lines,” J. Quant. Spectrosc. Radiat. Transf. 17(5), 681 – 684 (1977).
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M. Zadnik, S. Specht, and F. Begemann, “Revised isotopic composition of terrestrial mercury,” Int. J. Mass Spectrome. Ion Process. 89, 103 – 110 (1989).
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E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

Berengut, J. C.

J. C. Berengut, D. Budker, C. Delaunay, V. V. Flambaum, C. Frugiuele, E. Fuchs, C. Grojean, R. Harnik, R. Ozeri, G. Perez, and Y. Soreq, “Probing new long-range interactions by isotope shift spectroscopy,” Phys. Rev. Lett. 120, 091801 (2018).
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E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

Bielska, K.

N. Shiga, Y. Li, H. Ito, S. Nagano, T. Ido, K. Bielska, R. S. Trawiński, and R. Ciuryło, “Buffer-gas-induced collision shift for the  88Sr 1S 0−3P 1 clock transition,” Phys. Rev. A 80, 030501 (2009).
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J. K. Böhlke, J. R. De Laeter, P. De Bièvre, H. Hidaka, H. S. Peiser, K. J. R. Rosman, and P. D. P. Taylor, “Isotopic compositions of the elements, 2001,” J. Phys. Chem. Ref. Data 34(1), 57–67 (2005).
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E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

Drever, R. W. P.

R. W. P. Drever, J. L. Hall, F. V. Kowalski, J. Hough, G. M. Ford, A. J. Munley, and H. Ward, “Laser phase and frequency stabilization using an optical resonator,” Appl. Phys. B Photophysics Laser Chem. 31(2), 97–105 (1983).
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P. Morzyński, M. Bober, D. Bartoszek-Bober, J. Nawrocki, P. Krehlik, L. Śliwczyński, M. Lipiński, P. Masłowski, A. Cygan, P. Dunst, M. Garus, D. Lisak, J. Zachorowski, W. Gawlik, C. Radzewicz, R. Ciuryło, and M. Zawada, “Absolute measurement of the  1S 0 -  3P 0 clock transition in neutral  88Sr over the 330 km-long stabilized fibre optic link,” Sci. Rep. 5, 17495 (2015).
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Dzuba, V. A.

E. J. Angstmann, V. A. Dzuba, and V. V. Flambaum, “Relativistic effects in two valence-electron atoms and ions and the search for variation of the fine-structure constant,” Phys. Rev. A 70, 014102 (2004).
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Ellis, D. E.

E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

Erbert, G. V.

J. K. Crane, G. V. Erbert, S. D. Mostek, R. C. Kerlin, and J. A. Paisner, “High-resolution absorption spectrum of the 6 1S 0→6 3P 1 transition in mercury with a CW dye laser,” in AIP Conference Proceedings, (American Institute of Physics, 1986), pp. 411–412.

Flambaum, V. V.

V. V. Flambaum, A. J. Geddes, and A. V. Viatkina, “Isotope shift, nonlinearity of King plots, and the search for new particles,” Phys. Rev. A 97, 032510 (2018).
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J. C. Berengut, D. Budker, C. Delaunay, V. V. Flambaum, C. Frugiuele, E. Fuchs, C. Grojean, R. Harnik, R. Ozeri, G. Perez, and Y. Soreq, “Probing new long-range interactions by isotope shift spectroscopy,” Phys. Rev. Lett. 120, 091801 (2018).
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E. J. Angstmann, V. A. Dzuba, and V. V. Flambaum, “Relativistic effects in two valence-electron atoms and ions and the search for variation of the fine-structure constant,” Phys. Rev. A 70, 014102 (2004).
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Ford, G. M.

R. W. P. Drever, J. L. Hall, F. V. Kowalski, J. Hough, G. M. Ford, A. J. Munley, and H. Ward, “Laser phase and frequency stabilization using an optical resonator,” Appl. Phys. B Photophysics Laser Chem. 31(2), 97–105 (1983).
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Fortson, E. N.

M. D. Swallows, T. H. Loftus, W. C. Griffith, B. R. Heckel, E. N. Fortson, and M. V. Romalis, “Techniques used to search for a permanent electric dipole moment of the  199Hg atom and the implications for CP violation,” Phys. Rev. A 87, 012102 (2013).
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Fricke, B.

G. Torbohm, B. Fricke, and A. Rosén, “State-dependent volume isotope shifts of low-lying states of group-IIa and -IIb elements,” Phys. Rev. A 31(4), 2038–2053 (1985).
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M. L. Huber, A. Laesecke, and D. G. Friend, “Correlation for the vapor pressure of mercury,” Ind. Eng. Chem. Res. 45(21), 7351–7361 (2006).
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Frugiuele, C.

J. C. Berengut, D. Budker, C. Delaunay, V. V. Flambaum, C. Frugiuele, E. Fuchs, C. Grojean, R. Harnik, R. Ozeri, G. Perez, and Y. Soreq, “Probing new long-range interactions by isotope shift spectroscopy,” Phys. Rev. Lett. 120, 091801 (2018).
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Fuchs, E.

J. C. Berengut, D. Budker, C. Delaunay, V. V. Flambaum, C. Frugiuele, E. Fuchs, C. Grojean, R. Harnik, R. Ozeri, G. Perez, and Y. Soreq, “Probing new long-range interactions by isotope shift spectroscopy,” Phys. Rev. Lett. 120, 091801 (2018).
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Garus, M.

P. Morzyński, M. Bober, D. Bartoszek-Bober, J. Nawrocki, P. Krehlik, L. Śliwczyński, M. Lipiński, P. Masłowski, A. Cygan, P. Dunst, M. Garus, D. Lisak, J. Zachorowski, W. Gawlik, C. Radzewicz, R. Ciuryło, and M. Zawada, “Absolute measurement of the  1S 0 -  3P 0 clock transition in neutral  88Sr over the 330 km-long stabilized fibre optic link,” Sci. Rep. 5, 17495 (2015).
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Gawlik, W.

P. Morzyński, M. Bober, D. Bartoszek-Bober, J. Nawrocki, P. Krehlik, L. Śliwczyński, M. Lipiński, P. Masłowski, A. Cygan, P. Dunst, M. Garus, D. Lisak, J. Zachorowski, W. Gawlik, C. Radzewicz, R. Ciuryło, and M. Zawada, “Absolute measurement of the  1S 0 -  3P 0 clock transition in neutral  88Sr over the 330 km-long stabilized fibre optic link,” Sci. Rep. 5, 17495 (2015).
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P. Morzyński, P. Wcisło, P. Ablewski, R. Gartman, W. Gawlik, P. Masłowski, B. Nagórny, F. Ozimek, C. Radzewicz, M. Witkowski, R. Ciuryło, and M. Zawada, “Absolute frequency measurement of rubidium 5S - 7S two-photon transitions,” Opt. Lett. 38(22), 4581–4584 (2013).
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Geddes, A. J.

V. V. Flambaum, A. J. Geddes, and A. V. Viatkina, “Isotope shift, nonlinearity of King plots, and the search for new particles,” Phys. Rev. A 97, 032510 (2018).
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J. D. Deschênes and J. Genest, “Heterodyne beats between a continuous-wave laser and a frequency comb beyond the shot-noise limit of a single comb mode,” Phys. Rev. A 87, 023802 (2013).
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Ghysels, A.

E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

Giammona, A.

E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

Goez, A.

E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

Götz, A. W.

E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

Graner, B.

B. Graner, Y. Chen, E. G. Lindahl, and B. R. Heckel, “Reduced limit on the permanent electric dipole moment of  199Hg,” Phys. Rev. Lett. 116, 161601 (2016).
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Griffith, W. C.

M. D. Swallows, T. H. Loftus, W. C. Griffith, B. R. Heckel, E. N. Fortson, and M. V. Romalis, “Techniques used to search for a permanent electric dipole moment of the  199Hg atom and the implications for CP violation,” Phys. Rev. A 87, 012102 (2013).
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Grojean, C.

J. C. Berengut, D. Budker, C. Delaunay, V. V. Flambaum, C. Frugiuele, E. Fuchs, C. Grojean, R. Harnik, R. Ozeri, G. Perez, and Y. Soreq, “Probing new long-range interactions by isotope shift spectroscopy,” Phys. Rev. Lett. 120, 091801 (2018).
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Gusarov, S.

E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

Hachisu, H.

H. Hachisu, K. Miyagishi, S. G. Porsev, A. Derevianko, V. D. Ovsiannikov, V. G. Pal’chikov, M. Takamoto, and H. Katori, “Trapping of neutral mercury atoms and prospects for optical lattice clocks,” Phys. Rev. Lett. 100,053001 (2008).
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Hahn, A. A.

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P. L. Lee, F. Boehm, and A. A. Hahn, “Variations of nuclear charge radii in mercury isotopes with A=198, 199, 200, 201, 202, and 204 from x-ray isotope shifts,” Phys. Rev. C 17(5), 1859–1861 (1978).
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Hall, J. L.

M. D. Rayman, C. G. Aminoff, and J. L. Hall, “Precise laser frequency scanning using frequency-synthesized optical frequency sidebands: application to isotope shifts and hyperfine structure of mercury,” J. Opt. Soc. Am. B 6(4), 539–549 (1989).
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R. W. P. Drever, J. L. Hall, F. V. Kowalski, J. Hough, G. M. Ford, A. J. Munley, and H. Ward, “Laser phase and frequency stabilization using an optical resonator,” Appl. Phys. B Photophysics Laser Chem. 31(2), 97–105 (1983).
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Harnik, R.

J. C. Berengut, D. Budker, C. Delaunay, V. V. Flambaum, C. Frugiuele, E. Fuchs, C. Grojean, R. Harnik, R. Ozeri, G. Perez, and Y. Soreq, “Probing new long-range interactions by isotope shift spectroscopy,” Phys. Rev. Lett. 120, 091801 (2018).
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Harris, F. E.

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Porsev, S. G.

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Raczynski, A.

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Ramanantoanina, H.

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E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

van Lenthe, E.

E. van Lenthe, J. G. Snijders, and E. J. Baerends, “The zero-order regular approximation for relativistic effects: the effect of spin-orbit coupling in closed shell molecules,” J. Chem. Phys. 105(15), 6505–6516 (1996).
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E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

Van Meer, R.

S. Knecht, S. Fux, R. Van Meer, L. Visscher, M. Reiher, and T. Saue, “Mössbauer spectroscopy for heavy elements: a relativistic benchmark study of mercury,” Theor. Chem. Accounts 129(3–5), 631–650 (2011).
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E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

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E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

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S. Gerstenkorn, J. J. Labarthe, and J. Vergès, “Fine and hyperfine structures and isotope shifts in the arc spectrum of mercury. Part I. Experimental study of the infrared spectrum by Fourier transform spectroscopy,” Phys. Scripta 15(3), 167–172 (1977).
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E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

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E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

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C. J. Sansonetti and D. Veza, “Doppler-free measurement of the 546 nm line of mercury,” J. Phys. B: At. Mol. Opt. Phys. 43, 205003 (2010).
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V. V. Flambaum, A. J. Geddes, and A. V. Viatkina, “Isotope shift, nonlinearity of King plots, and the search for new particles,” Phys. Rev. A 97, 032510 (2018).
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Villwock, P.

P. Villwock, S. Siol, and T. Walther, “Magneto-optical trapping of neutral mercury,” The Eur. Phys. J. D 65(1), 251–255 (2011).
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S. Knecht, S. Fux, R. Van Meer, L. Visscher, M. Reiher, and T. Saue, “Mössbauer spectroscopy for heavy elements: a relativistic benchmark study of mercury,” Theor. Chem. Accounts 129(3–5), 631–650 (2011).
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E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

Walter, H. K.

A. A. Hahn, J. P. Miller, R. J. Powers, A. Zehnder, A. M. Rushton, R. E. Welsh, A. R. Kunselman, P. Roberson, and H. K. Walter, “An experimental study of muonic x-ray transitions in mercury isotopes,” Nucl. Phys. A 314(2–3), 361–386 (1979).
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Walther, T.

P. Villwock, S. Siol, and T. Walther, “Magneto-optical trapping of neutral mercury,” The Eur. Phys. J. D 65(1), 251–255 (2011).
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E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

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R. W. P. Drever, J. L. Hall, F. V. Kowalski, J. Hough, G. M. Ford, A. J. Munley, and H. Ward, “Laser phase and frequency stabilization using an optical resonator,” Appl. Phys. B Photophysics Laser Chem. 31(2), 97–105 (1983).
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Welsh, R. E.

A. A. Hahn, J. P. Miller, R. J. Powers, A. Zehnder, A. M. Rushton, R. E. Welsh, A. R. Kunselman, P. Roberson, and H. K. Walter, “An experimental study of muonic x-ray transitions in mercury isotopes,” Nucl. Phys. A 314(2–3), 361–386 (1979).
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Wendt, K.

G. Ulm, S. K. Bhattacherjee, P. Dabkiewicz, G. Huber, H. J. Kluge, T. Kühl, H. Lochmann, E. W. Otten, K. Wendt, S. A. Ahmad, W. Klempt, R. Neugart, and ISOLDE Collaboration, “Isotope shift of  182Hg and an update of nuclear moments and charge radii in the isotope range  181Hg- 206Hg,” Zeitschrift für Physik A Atomic Nuclei 325(3), 247–259 (1986).
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E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

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E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

Witkowski, M.

Wolff, S. K.

E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

Woo, T. K.

E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

Yakovlev, A. L.

E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

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Zawada, M.

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E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

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M. Witkowski, R. Munoz-Rodriguez, A. Raczyński, J. Zaremba, B. Nagórny, P. S. Żuchowski, R. Ciuryło, and M. Zawada, “Photoionization cross section of the  5S 1/2 and  5P 3/2 states of Rb in simultaneous magneto-optical trapping of Rb and Hg,” Phys. Rev. A 98, 053444 (2018).
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E. J. Baerends, T. Ziegler, A. J. Atkins, J. Autschbach, D. Bashford, O. Baseggio, A. Bérces, F. M. Bickelhaupt, C. Bo, P. M. Boerritger, L. Cavallo, C. Daul, D. P. Chong, D. V. Chulhai, L. Deng, R. M. Dickson, J. M. Dieterich, D. E. Ellis, M. van Faassen, A. Ghysels, A. Giammona, S. J. A. van Gisbergen, A. Goez, A. W. Götz, S. Gusarov, F. E. Harris, P. van den Hoek, Z. Hu, C. R. Jacob, H. Jacobsen, L. Jensen, L. Joubert, J. W. Kaminski, G. van Kessel, C. König, F. Kootstra, A. Kovalenko, M. Krykunov, E. van Lenthe, D. A. McCormack, A. Michalak, M. Mitoraj, S. M. Morton, J. Neugebauer, V. P. Nicu, L. Noodleman, V. P. Osinga, S. Patchkovskii, M. Pavanello, C. A. Peeples, P. H. T. Philipsen, D. Post, C. C. Pye, H. Ramanantoanina, P. Ramos, W. Ravenek, J. I. Rodríguez, P. Ros, R. Rüger, P. R. T. Schipper, D. Schlüns, H. van Schoot, G. Schreckenbach, J. S. Seldenthuis, M. Seth, J. G. Snijders, M. Solà, M. Stener, M. Swart, D. Swerhone, G. te Velde, V. Tognetti, P. Vernooijs, L. Versluis, L. Visscher, O. Visser, F. Wang, T. A. Wesolowski, E. M. van Wezenbeek, G. Wiesenekker, S. K. Wolff, T. K. Woo, and A. L. Yakovlev, “ADF2017, SCM, Theoretical Chemistry, Vrije Universiteit, Amsterdam, The Netherlands,” (2017).

A. Unsöld, Physik der Sternatmosphären (Springer, 1955).
[Crossref]

C. E. Moore, Atomic Energy Levels, vol. 3 (U.S. Government Printing Office, 1958).

J. Reader, C. H. Corliss, W. L. Wiese, and G. A. Martin, Wavelengths and transition probabilities for atoms and atomic ion (U.S. Government Printing Office, 1980).

W. H. King, Isotope Shifts in Atomic Spectra (Springer, 1984).
[Crossref]

J. R. Paul, “Construction and characterization of a neutral Hg magneto-optical trap and precision spectroscopy of the 61P0 – 63P0 Hg199 clock transition,” Ph.D. thesis, The University of Arizona (2015).

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Figures (9)

Fig. 1
Fig. 1 A simplified scheme of the laser setup. A fourth harmonic generation laser system delivers up to 30 mW of the 253.7 nm laser light which is frequency shifted by a double-pass transition in the acousto-optical modulator AOM1 and then directed to a mercury cell. A Doppler-free saturation absorption signal is used to monitor a deviation of the UV laser frequency from an atomic transition of a given Hg isotope. A part of the 1014.8 nm laser light is transferred through an AOM2 to a transfer cavity. The cavity length is stabilized to the wavelength of a 689 nm laser while the 1014.8 nm laser wavelength is locked to one of the cavity modes. The frequency of the 1014.8 nm laser is compared via the optical frequency comb to the frequencies of UTC(AOS) and UTC(PL) [29, 30] via the stabilized fibre optic link [31] of the OPTIME network [32, 33]. DDS stands for a direct digital synthesizer, PC – a desktop computer, μ-c – a microcontroller, PD – a photodiode, and PDH – Pound-Drever-Hall locking technique.
Fig. 2
Fig. 2 Schematic illustration of the background-induced frequency shift of the typical saturated absorption spectral line. a) a symmetrical profile; the red solid curve shows the slope-dependent SNR in the digital locking technique. b) a profile with a linear background. c) a profile with a linear (grey) and a non-linear (black) background. The red (panel b) and green (panel c) circles correspond to the probed range 2δf in the linear and the non-linear background case, respectively. The inflection points of the profile are marked with the blue circles. f0 (blue arrow) is a non-shifted frequency, fSNR (red arrow) and fSNR+NL (green arrow) are the frequencies obtained with f+ and f calculated from maximal SNR of fUV signal with the linear and the non-linear background, respectively.
Fig. 3
Fig. 3 Top: structure of the 254 nm line in the natural isotopic composition of mercury based on the data published by Schweitzer [35] and Zadnik [36]. Red and blue colour corresponds to bosons and fermions, respectively. The letters indicate the following hyperfine components: F = 1/2 (a), F = 3/2 (b), and F = 5/2 (c). The line strengths are normalized to the most abundant isotope, i.e. 202Hg. Bottom: a typical saturated absorption spectroscopy signal recorded in our measurements, averaged about ten times and power broadened for better visibility.
Fig. 4
Fig. 4 A scheme of the relevant frequencies, both radio (denoted by f) and optical (denoted by ν), used in the experimental setup. The coloured arrows indicate schematic paths of the laser beams while the black arrows correspond to the RF signalssent to a PC-based data acquisition system.
Fig. 5
Fig. 5 Results of the absolute frequency measurements for 1S03P1 transition in Hg isotopes. Both sample standard deviation (red error bars) and mean standard deviation (black error bars) for a given measurement are shown. The red dotted lines and the blue dashed lines are statistical and total (including statistical and systematic) uncertainties, respectively, as listed in Table 2.
Fig. 6
Fig. 6 Results of a sample AC-Stark shift measurement in the 1S0-3P1 transition of 204Hg. f204Hg is the absolute frequency of the transition. Each point represents the average of measurements for a given power of the UV light. Black and red error bars correspond to the mean and the sample standard deviation, respectively. The dashed blue lines indicate linear regression bands. The black solid line is the linear regression fit to the data weighted by the mean standard deviations.
Fig. 7
Fig. 7 Comparison of present work results to the previous determinations of the 1S03P1 frequency for different Hg isotopes. The experimental results are referenced to the following lines: 198Hg 546 nm (green circle), 86Kr 606 nm (red square) and 198Hg 185 nm (blue triangle). (1), (2) Burns and Adams [49, 50], (3) Gerstenkorn et al. eGerstenkorn1977, (4) Meggers and Kessler [52], (5) Barger and Kessler [53], (6) Barger and Kessler result corrected according to the Bruce and Hill data [54], (7) correction of the Barger result [53] made by Kramida [9] based on the measurement of 313.2749895 nm 198Hg [55] as a reference, (8) Kaufman [56], (9) Schweitzer [35], (10) Schweitzer’s result [35] corrected according to the Bruce and Hill data [54]. Black points are our results while the orange ones (cross) correspond to the corrected measurements.
Fig. 8
Fig. 8 A comparison of isotope shift results referenced to 198Hg. Our results (black) are compared with the data shown by Schweitzer [35] (blue circle), Crane [57] (red cross) and Gerstenkorn [51] (brown square). For better visibility, the results are separated horizontally and shifted by an isotope shift value measured in the present work for a given isotope.
Fig. 9
Fig. 9 King plot of normalised isotope shifts in the 6s6p 3P2-6s7s 3S1 (546 nm) transition (taken from [24]) versus normalised isotope shifts in the 5d10 6s2 1S0-5d10 6s6p 3P1 (254 nm) transition (our results). The isotope shifts of 199Hg were shifted to the centre of gravity of the hyperfine manifold according to the data published by Rayman [24], Sansonetti [58] (546 nm), and Stager [59] (254 nm). The red solid line is the linear fit weighted by uncertainties of isotope shifts. The common reference isotope is 198Hg.

Tables (3)

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Table 1 Systematic shifts and their uncertainties for typical experimental conditions, i.e. the UV laser beam intensity of 400 W/m2 and the temperature of the Hg-vapour cell of 26.1°C. All results are in MHz. Remote frequency reference characterisation, i.e. gravitational red shift between AOS laboratory and our laboratory as well as uncertainty between UTC(AOS) and TT (the SI second on the geoid) are taken from [31].

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Table 2 Measured absolute frequencies of the 1S0-3P1 transition.

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Table 3 Isotope shifts for the 1S0-3P1 transition in Hg referenced to 198Hg. The measured values are compared with the results presented by Schweitzer [35], Crane [57] and Gerstenkorn [51].

Equations (4)

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f U V = 4 ( f o + n f R ± f B 2 f A O M 2 ) + 2 f A O M 1 ,
I S i A A = A A A A M S i + E i δ r 2 A A ,
ζ 546 A A = ζ 254 A A E 546 E 254 + M S 546 E 546 E 254 M S 254 .
E i = Z e 2 6 ϵ 0 Δ ρ el ( 0 ) ,

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